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PubMed1986

A Monte Carlo program to calculate the exposure rate from airborne radioactive gases inside a nuclear reactor containment building.

A program was developed to calculate the exposure rate resulting from airborne gases inside a reactor containment building. The calculations were performed at the location of a wall-mounted area radiation monitor. The program uses Monte Carlo techniques and accounts for both the direct and scattered components of the radiation field at the detector. The scattered component was found to contribute about 30% of the total exposure rate at 50 keV and dropped to about 7% at 2000 keV. The results of the calculations were normalized to unit activity per unit volume of air in the containment. This allows the exposure rate readings of the area monitor to be used to estimate the airborne activity in containment in the early phases of an accident. Such estimates, coupled with containment leak rates, provide a method to obtain a release rate for use in offsite dose projection calculations.

Accidents↗
PubMed1990

Adsorption and desorption of noble gases on activated charcoal: I. 133Xe studies in a monolayer and packed bed.

Detailed desorption studies using petroleum-based activated charcoals were conducted in monolayers and packed beds. Less extensive studies were conducted on several other types of charcoal. Kinetic studies, using 133Xe, demonstrated the existence of a micropore volume with entrance capillaries that together determined the response characteristics of charcoal to external concentration gradients of tracer gases. This new two-phase model, composed of micropores and entrance capillaries, describes the desorption dynamics of an adsorbed gas in the presence of water vapor. Condensed water vapor in the entrance capillaries of the charcoal reduced the effective pore radius and increased the diffusion half-time. Water could also adversely affect the integrating capability of the charcoal dramatically if the adsorbed water completely blocked the entrance capillaries. The amount of adsorbed water required to block the capillaries varied with the charcoal type and was termed here as the "break-point." The desorption parameters measured in this work can be used to design an improved passive Rn monitor to effectively integrate during a 3-7 d exposure period by eliminating the adverse effects of water vapor. The improved canister design would provide more accurate and reproducible measurements of indoor Rn concentrations than are currently available.

Adsorption↗
PubMed1991

Radioiodine speciation in the hot cell effluent gases of a radiopharmaceutical production facility.

In order to characterize the various chemical forms of airborne radioiodine species, grab-sampling measurements were conducted at the hot cell laboratory of a radiopharmaceutical production facility, using a selective-adsorbent-iodine filter system. Volatile radioiodine species were produced in the hot cell process which extracted the fission product 99Mo from the irradiated uranium target. The effluent gases were then released through the hot cell filter bank and the main filter bank. Two samplings were made, one at the inlet and one at the outlet of the hot cell filter bank. In comparison with other radioiodine isotopes detected, higher than expected concentrations of 132I were found, primarily in the form of organic iodide--an observation that could be explained by the beta decay of 132Te, the precursor of 132I, in the hot cell waste solution. The relative distribution of airborne 132I was considerably different from that of other iodine radioisotopes. An unexpected component of these distributions was radioiodine penetrating the silver zeolite filter and adsorbed on a triethylenediamine (TEDA) impregnated charcoal filter.

Air Pollutants, Radioactive↗
PubMed1994

Neutralization of thoron progeny in gases.

This paper reports charge neutralization phenomena of 212Pb particles in nitrogen or oxygen atmospheres with trace amounts of other gases. Newly produced thoron or radon progeny are positively charged, stable molecular clusters that are subsequently neutralized by several mechanisms. The charged clusters have a smaller diffusion coefficient than neutral clusters of the same size due to the interaction of the charge with the surrounding gas molecules. In this study, we have found that the diffusion coefficients of 212Pb in O2, N2, NH3/O2, NH3/N2, and C6H12/N2 (IPs between 15.58 and 9.8 eV) ranged between 0.015 and 0.030 cm2 s-1. In the case of C6H12/O2, NO2/O2, NO/O2, and dimethylamine/O2 (ionization potential between 9.8 and 8.23 eV), the diffusion coefficients have increased to between 0.046 and 0.69 cm2 s-1. These results are consistent with previous results of 218Po, indicating that charged progeny are neutralized by electron transfer from a gas molecule with a lower ionization potential than lead oxide. We estimate the ionization potential of lead oxide to range between 9.8 and 10.2 eV. 212Pb was also neutralized by an electron scavenging mechanism in NO2/nitrogen.

Air Pollution, Radioactive↗
PubMed1997

Brain tissue gases and pH during arteriovenous malformation resection.

OBJECTIVE: The purpose of this study was to determine whether baseline partial pressure of oxygen (PO2), partial carbon dioxide pressure (PCO2), and pH in brain tissue adjacent to arteriovenous malformations (AVMs) are different from those in control patients. In addition, PO2, PCO2, and pH changes were measured during resection of the AVMs. METHODS: Two groups were studied. Group 1 (n = 8) was composed of nonischemic patients scheduled for cerebral aneurysm clipping. Group 2 (n = 13) was composed of patients undergoing neurosurgery for resection of AVMs. After the craniotomy, the dura was retracted and a combined PO2, PCO2, and pH sensor was inserted into nonischemic brain tissue in Group 1. In Group 2, the sensor was inserted into tissue 2 to 3 cm from the margin of the AVMs, within the same arterial blood supply. After equilibration of the sensor, tissue gases and pH were measured during steady-state anesthetic conditions in Group 1 and during resection of AVMs in Group 2. RESULTS: Under baseline conditions before the start of surgery, tissue PO2 was decreased in patients with AVMs compared with control patients, but PCO2 and pH were not changed. During resection of the AVMs, PO2 and pH increased and PCO2 decreased compared with baseline measurements. These parameters did not change in control patients during a similar time period. CONCLUSION: The results suggest that cerebrovascular or metabolic adaptation occurs in patients with AVMs with decreased tissue perfusion pressure as an adjustment for decreased oxygen delivery. During resection of AVMs, this adaptation produces a relative hyperemic environment with tissue hyperoxia, hypocapnia, and alkalosis that is not corrected by the end of surgery.

Acid-Base Equilibrium↗
PubMed2006

Clustered gases as a medium for efficient plasma waveguide generation.

Clustered gas jets are shown to be an efficient means for plasma waveguide generation, for both femtosecond and picosecond generation pulses. These waveguides enable significantly lower on-axis plasma density (less than 10(18) cm(-3)) than in conventional hydrodynamic plasma waveguides generated in unclustered gases. Using femtosecond pump pulses, self-guided propagation and strong absorption (more than 70%) are used to produce long centimetre scale channels in an argon cluster jet, and a subsequent intense pulse is coupled into the guide with 50% efficiency and guided at above 10(17)W cm(-2) intensity over 40 Rayleigh lengths. We also demonstrate efficient generation of waveguides using 100 ps axicon-generated Bessel-beam pump pulses. Despite the expected sub-picosecond cluster disassembly time, we observe long pulse absorption efficiencies up to a maximum of 35%. Simulations show that in the far leading edge of the long laser pulse, the volume of heated clusters evolves to a locally uniform and cool plasma already near ionization saturation, which is then efficiently heated by the remainder of the pulse.

Journal Article↗
PubMed1999

Onsager-Casimir reciprocity relation for the gyrothermal effect with polyatomic gases.

On the basis of the linearized Boltzmann equation and the boundary condition for the distribution function, the Onsager-Casimir reciprocity relation is derived for polyatomic gases confined between two cylinders in the presence of a magnetic field. The cross effect, namely, the heat flux caused by the rotation of the inner cylinder is predicted. Because of the heat flux the cylinder can be heated or cooled depending on the direction of the magnetic field. This effect is coupled with the gyrothermal effect by the reciprocity relation.

Journal Article↗
PubMed1999

Diffusion in lattice Lorentz gases with a percolation threshold.

A mean-field approximation for the diffusion coefficient in lattice Lorentz gases with an arbitrary mixture of pointlike stochastic scatterers in the low-density limit is proposed. In this approximation, the diffusion coefficient is directly related to the first return probability of the moving particle in the corresponding Cayley tree through an effective ring operator. A renormalization scheme for the approximate determination of the first return probability is constructed. The predictions of this mean-field theory and those of the repeated ring approximation (RRA) are compared with computer simulation results for models in which a fraction x(B) of the scatterers are deterministic backscatterers, so that the diffusion coefficient vanishes beyond a certain percolation threshold x(c)(B). The approximation proposed in this paper is seen to be in good agreement with the simulation results, in contrast to the RRA, which already fails to give the correct percolation threshold.

Journal Article↗
PubMed2000

Renormalized field theory of driven lattice gases under infinitely fast drive

We use field theoretic renormalization group methods to study the critical behavior of a recently proposed Langevin equation for driven lattice gases under infinitely fast drive. We perform an expansion around the upper critical dimension, d(c)=4, and obtain the critical exponents to one-loop order. The main features of the two-loop calculation are also outlined. The renormalized theory is shown to exhibit a behavior different from the standard field theory for the driven lattice gas with finite driving, i.e., it is not mean-field-like.

Journal Article↗
PubMed2000

Logarithmically slow expansion of hot bubbles in gases

We predict a logarithmically slow expansion of hot bubbles in gases in the process of cooling. A model problem is first solved, when the temperature has compact support. Then the temperature profile decaying exponentially at large distances is considered. The periphery of the bubble is shown to remain essentially static ("glassy") in the process of cooling until it is taken over by a logarithmically slowly expanding "core." An analytical solution to the problem is obtained by matched asymptotic expansion. This problem gives an example of how logarithmic corrections enter dynamic scaling.

Journal Article↗
PubMed2000

Theory of collision algorithms for gases and plasmas based on the boltzmann equation and the landau-fokker-planck equation

A time-explicit formula that describes the time evolution of velocity distribution functions of gases and plasmas is derived from the Boltzmann equation. The formula can be used to construct collision simulation algorithms. Specialization of the formula to the case of the Coulomb interaction shows that the previous method [K. Nanbu, Phys. Rev. E 55, 4642 (1997)] for a Coulomb collision simulation is a solution method of the Landau-Fokker-Planck equation in the limit of a small time step. Also, a collision simulation algorithm for multicomponent plasmas is proposed based on the time-explicit formula derived.

Journal Article↗
PubMed2000

Universality classes of driven lattice gases

Motivated by some recent criticisms to our alternative Langevin equation for driven lattice gases (DLG) under an infinitely large driving field, we revisit the derivation of such an equation, and test its validity. As a result, an additional term, coming from a careful consideration of entropic contributions, is added to the equation. This term heals all the recently reported generic infrared singularities. The emerging equation is then identical to that describing randomly driven diffusive systems. This fact confirms our claim that the infinite driving limit is singular, and that the main relevant ingredient determining the critical behavior of the DLG in this limit is the anisotropy and not the presence of a current. Different aspects of our picture are discussed, and it is concluded that it constitutes a very plausible scenario to rationalize the critical behavior of the DLG and variants of it.

Journal Article↗
PubMed2000

Modeling of gas dynamics for a laser-generated plasma: propagation into low-pressure gases

The physical phenomena involved during three-dimensional axisymmetric laser-induced plasma expansion into background gas are numerically studied. For this purpose, a multispecies hydrodynamic model is developed which considers the effects of mass and ambipolar diffusions, thermal conduction, viscosity, and nonequilibrium conditions for ionization. This model is applied to describe quantitatively the Si plasma plume expansion into Ar or He gases. It is shown that the mechanism of plasma expansion depends critically on both the pressure and mass of the background gas. The shock front expansion is found to be strongly correlated with ion dynamics. A pronounced difference between heavy-particle and electron temperatures indicates a persistent lack of equilibrium between the heavy particle and the electron in the plasma plume expansion. The Si atoms of the rarefied plume are essentially driven by the backward-moving background gas as a result of a mass diffusion process. It is also noted that the diffusion processes are only important in the last expansion stage, and are less significant in the first stage. Therefore, it is shown that a computation which does not include diffusion effects (Euler equations) can adequately describe only the earliest stage of plasma expansion into background gas. The ability of the Navier-Stokes hydrodynamic multispecies model to predict the key role of the background gas type (Ar, He) and pressure is demonstrated.

Journal Article↗
PubMed2000

Effect of boundary conditions on diffusion in two-dimensional granular gases.

We analyze the influence of boundary conditions on numerical simulations of the diffusive properties of a two-dimensional granular gas. We show in particular that periodic boundary conditions introduce unphysical correlations in time that cause the coefficient of diffusion to be strongly dependent on the system size. On the other hand, in large enough systems with hard walls at the boundaries, diffusion is found to be independent of the system size. We compare the results obtained in this case with Langevin theory for an elastic gas. Good agreement is found. We then calculate the relaxation time and the influence of the mass for a particle of radius R(s) in a sea of particles of radius R(b). As granular gases are dissipative, we also study the influence of an external random force on the diffusion process in a forced dissipative system. In particular, we analyze differences in the mean-square velocity and displacement between the elastic and inelastic cases.

Journal Article↗
PubMed2001

Extremal principle for the steady-state selection in driven lattice gases with open boundaries.

This paper investigates the steady states of one-dimensional driven lattice gases with open boundary conditions. It shows how the extremal principle proposed recently by Popkov and Schütz can be modified to apply to more general cases. Monte Carlo simulations are presented for a one-dimensional totally asymmetric simple exclusion process with nearest neighbor repulsion under parallel update as an example. The simulations enable one to guess the exact phase diagram for this particular lattice gas with deterministic bulk dynamics, by fitting the data to analytic formulas, which appear to be exact in the thermodynamic limit.

Journal Article↗
PubMed2001

Driven granular gases with gravity.

We study fluidized granular gases in a stationary state determined by the balance between external driving and bulk dissipation. The two considered situations are inspired by recent experiments, where gravity plays a major role as a driving mechanism: in the first case, gravity acts only in one direction and the bottom wall is vibrated; in the second case, gravity acts in both directions and no vibrating walls are present. Simulations performed under the molecular chaos assumption show averaged profiles of density, velocity, and granular temperature that are in good agreement with the experiments. Moreover, we measure velocity distributions that show strong non-Gaussian behavior, as experiments pointed out, but also density correlations accounting for clustering, at odds with the experimental results. The hydrodynamics of the first model is discussed and an exact solution is found for the density and granular temperature as functions of the distance from the vibrating wall. The limitations of such a solution, in particular in a broad layer near the wall injecting energy, are discussed.

Journal Article↗
PubMed2002

Correlation functions in classical gases at high frequency.

A general procedure is outlined to determine the exact asymptotic form of spectra in classical gases at high frequency. Examples are the force-force correlation or the velocity autocorrelation function of a tagged particle. For purely repulsive potentials of the form Ar(-n), the asymptotic spectra are proportional to omega(sigma)exp[-(omegatau)(nu)]. Exponent nu and time constant tau depend only on the interparticle potential, while exponent sigma depends in addition on the correlation studied. The analysis makes use of the fact that the high-frequency spectra are dominated by high-energy binary collisions. It is argued that for arbitrary potentials the spectra decay slower than exp(-constxomega(2/3)) and that the results are also relevant for dense fluids. The frequency range is estimated where quantum effects become important.

Journal Article↗