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At least 469 records · Page 26Linked to original sources
PubMed1984

Mechanism of phosphine photolysis. Application to Jovian atmospheric photochemistry.

PH3 is photolyzed to H2 and P2H4 and the P2H4 in turn is converted to red phosphorus. The initial quantum yield of H2 formation was redetermined and found to be 0.93 +/- 0.07. Red phosphorus was identified by its chemical properties and the absence of P-H stretching bands in its infrared spectrum. The reaction pathway was not changed by lowering the PH3 partial pressure from 90 to 11 torr or by performing the photolysis in a 70-fold excess of H2. The initial quantum yields at 11 torr of PH3 are phi P2H4 = 0.04 +/- 0.02 and phi H2 = 0.74 +/- 0.08. The initial rate of P2H4 formation was not affected by lowering the PH3 temperature to 227 or 157 K. The yield was greater at 157 K because the P2H4 condensed and was protected from further destruction. The initial quantum yields for the formation of P2H4 and H2 in PH3-NH3 mixtures were comparable to those observed for PH3 alone. Photolysis of mixtures in which NH3 was absorbing 90% of the light resulted in the rapid formation of P2H4. No N2 was formed when PH3-NH3 mixtures were photolyzed, suggesting that the destruction of NH3 is quenched by PH3. The application of these findings to Jovian atmospheric chemistry is discussed.

Ammonia↗
PubMed1998

A search for extraterrestrial eukaryotes: physical and paleontological aspects.

Physical and biochemical aspects of a proposed search for extraterrestrial eukaryotes (SETE) are considered. Such a program should approach the distinction between a primitive eukaryote and an archaebacteria. The emphasis on gene silencing suggests a possible assay suitable for a robotic investigation of eukaryoticity, so as to be able to decide whether the first steps towards eukaryogenesis have been taken in an extraterrestrial planet, or satellite. The experiment would consist of searching for cellular division and the systematic related delay in replication of heterochromatic chromosome segments. It should be noticed that the direct search for a membrane-bounded set of chromosomes does not necessarily determine eukaryotic identity, as there are prokaryotes that have membrane-bounded nucleoids. A closer look at the protein fraction of chromatin (mainly histones) does not help either, as there are some eukaryotes that may lack histones; there are also some bacteria as well as archaebacteria with histone-like proteins in their nucleoids. Comments on the recent suggestion of possible environments for a SETE program are discussed: the deep crust of Mars, and the Jovian satellite Europa, provided the existence of an ocean under its ice-covered surface is confirmed by the current Galileo mission.

Biological Evolution↗
PubMed2002

Europa as an abode of life.

Life as we know it on Earth depends on liquid water, a suite of 'biogenic' elements (most famously carbon) and a useful source of free energy. Here we review Europa's suitability for life from the perspective of these three requirements. It is likely, though not yet certain, that Europa harbors a subsurface ocean of liquid water whose volume is about twice that of Earth's oceans. Little is known about Europa's inventory of carbon, nitrogen, and other biogenic elements, but lower bounds on these can be placed by considering the role of commentary delivery over Europa's history. Sources of free energy are challenging for a world covered with an ice layer kilometers thick, but it is possible that hydrothermal activity and/or organics and oxidants provided by the action of radiation chemistry at Europa's surface and subsequent mixing into Europa's ocean could provide the electron donors and acceptors needed to power a Europan ecosystem. It is not premature to draw lessons from the search for life on Mars with the Viking spacecraft for planning exobiological missions to Europa.

Carbon↗
PubMed1995

Influx of cometary volatiles to planetary moons: the atmospheres of 1000 possible Titans.

We use a Monte Carlo model to simulate impact histories of possible Titans, Callistos, and Ganymedes. Comets create or erode satellite atmospheres, depending on their mass and velocity distributions: faster and bigger comets remove atmophiles; slower or smaller comets supply them. Mass distributions and the minimum total mass of comets passing through the Saturn system were derived from the crater records of Rhea and Iapetus. These were then scaled to give a minimum impact history for Titan. From this cometary population, of 1000 initially airless Titans, 16% acquired atmospheres larger than Titan's present atmosphere (9 x 10(21) g), and more than half accumulated atmospheres larger than 10(21) g. In contrasts to the work of Zahnle et al. (1992), we find that, in most trials, Callisto acquires comet-based atmospheres. Atmospheres acquired by Callisto and, especially, Ganymede are sensitive to assumptions regarding energy partitioning into the ejecta plume. If we assume that only the normal velocity component heats the plume, the majority of Ganymedes and half of the Callistos accreted atmospheres smaller than 10(20) g. If all the impactor's velocity heats the plume, Callisto's most likely atmosphere is 10(17) g and Ganymede's is negligible. The true cometary flux was most likely larger than that derived from crater records, which raises the probability that Titan, Ganymede, and Callisto acquired substantial atmospheres. However, other loss processes (e.g., sputtering by ions swept up by the planetary magnetic field, solar UV photolysis of hydrocarbons) are potentially capable of eliminating small atmospheres over the age of the solar system. The dark material on Callisto's surface may be a remnant of an earlier, now vanished atmosphere.

Atmosphere↗
PubMed1998

The composition of the Jovian atmosphere as determined by the Galileo probe mass spectrometer.

The Galileo probe mass spectrometer determined the composition of the Jovian atmosphere for species with masses between 2 and 150 amu from 0.5 to 21.1 bars. This paper presents the results of analysis of some of the constituents detected: H2, He, Ne, Ar, Kr, Xe, CH4, NH3, H2O, H2S, C2 and C3 nonmethane hydrocarbons, and possibly PH3 and Cl. 4He/H2 in the Jovian atmosphere was measured to be 0.157 +/- 0.030. 13C/C12 was found to be 0.0108 +/- 0.0005, and D/H and 3He/4He were measured. Ne was depleted, < or = 0.13 times solar, Ar < or = 1.7 solar, Kr < or = 5 solar, and Xe < or = 5 solar. CH4 has a constant mixing ratio of (2.1 +/- 0.4) x 10(-3) (12C, 2.9 solar), where the mixing ratio is relative to H2. Upper limits to the H2O mixing ratio rose from 8 x 10(-7) at pressures <3.8 bars to (5.6 +/- 2.5) x 10(-5) (16O, 0.033 +/- 0.015 solar) at 11.7 bars and, provisionally, about an order of magnitude larger at 18.7 bars. The mixing ratio of H2S was <10(-6) at pressures less than 3.8 bars but rose from about 0.7 x 10(-5) at 8.7 bars to about 7.7 x 10(-5) (32S, 2.5 solar) above 15 bars. Only very large upper limits to the NH3 mixing ratio have been set at present. If PH3 and Cl were present, their mixing ratios also increased with pressure. Species were detected at mass peaks appropriate for C2 and C3 hydrocarbons. It is not yet clear which of these were atmospheric constituents and which were instrumentally generated. These measurements imply (1) fractionation of 4He, (2) a local, altitude-dependent depletion of condensables, probably because the probe entered the descending arm of a circulation cell, (3) that icy planetesimals made significant contributions to the volatile inventory, and (4) a moderate decrease in D/H but no detectable change in (D + 3He)/H in this part of the galaxy during the past 4.6 Gyr.

Atmosphere↗
PubMed1998

The biological potential of Mars, the early Earth, and Europa.

The potential biomass that could have existed on Mars is constrained by the total amount of energy available to construct it. From an inventory of the available geochemical sources of energy, we estimate that from the time of the onset of the visible geologic record 4 b.y. ago to the present, as much as 20 g cm-2 of biota could have been created. This is the same amount that could have been constructed on the early Earth in only 100 million years. This indicates that there likely was sufficient energy available to support an origin of life on Mars but not sufficient energy to create a ubiquitous and lush biosphere. Similar calculations for Europa suggest that even less would have been available there.

Biomass↗
PubMed1998

Production of O2 on icy satellites by electronic excitation of low-temperature water ice.

The signature of condensed molecular oxygen has been reported in recent optical-reflectance measurements of the jovian moon Ganymede, and a tenuous oxygen atmosphere has been observed on Europa. The surfaces of these moons contain large amounts of water ice, and it is thought that O2 is formed by the sputtering of ice by energetic particles from the jovian magnetosphere. Understanding how O2 might be formed from low-temperature ice is crucial for theoretical and experimental simulations of the surfaces and atmospheres of icy bodies in the Solar System. Here we report laboratory measurements of the threshold energy, cross-section and temperature dependence of O2 production by electronic excitation of ice in vacuum, following electron-beam irradiation. Molecular oxygen is formed by direct excitation and dissociation of a stable precursor molecule, rather than (as has been previously thought) by diffusion and chemical recombination of precursor fragments. The large cross-section for O2 production suggests that electronic excitation plays an important part in the formation of O2 on Ganymede and Europa.

Cold Temperature↗
PubMed1986

Deuterium in the outer Solar System: evidence for two distinct reservoirs.

We have just completed a series of determinations of the CH3D/CH4 ratio in the atmospheres of Saturn, Titan and Uranus. These results, coupled with the work of other investigators, suggest that the Solar System contains at least two distinctly different primordial reservoirs of deuterium: that contained in gaseous hydrogen and that contained in the volatiles which have been maintained at low temperatures or isolated from hydrogen; for example, trapped in cold, solid material. Both of these reservoirs were established before the formation of the Solar System.

Atmosphere↗
PubMed1998

Episodic plate separation and fracture infill on the surface of Europa. Galileo Imaging Team.

Images obtained by the Voyager spacecraft revealed dark, wedge-shaped bands on Europa that were interpreted as evidence that surface plates, 50-100 km across, moved and rotated relative to each other. This implied that they may be mechanically decoupled from the interior by a layer of warm ice or liquid water. Here we report similar features seen in higher resolution images (420 metres per pixel) obtained by the Galileo spacecraft that reveal new details of wedge-band formation. In particular, the interior of one dark band shows bilateral symmetry of parallel lineaments and pit complexes which indicates that plate separation occurred in discrete episodes from a central axis. The images also show that this style of tectonic activity involved plates < 10 km across. Although this tectonic style superficially resembles aspects of similar activity on Earth, such as sea-floor spreading and the formation of ice leads in polar seas, there are significant differences in the underlying physical mechanisms: the wedge-shaped bands on Europa most probably formed when lower material (ice or water) rose to fill the fractures that widened in response to regional surface stresses.

Geological Phenomena↗
PubMed2001

Flooding of Ganymede's bright terrains by low-viscosity water-ice lavas.

Large regions of the jovian moon Ganymede have been resurfaced, but the means has been unclear. Suggestions have ranged from volcanic eruptions of liquid water or solid ice to tectonic deformation, but definitive high-resolution morphological evidence has been lacking. Here we report digital elevation models of parts of the surface of Ganymede, derived from stereo pairs combining data from the Voyager and Galileo spacecraft, which reveal bright, smooth terrains that lie at roughly constant elevations 100 to 1,000 metres below the surrounding rougher terrains. These topographic data, together with new images that show fine-scale embayment and burial of older features, indicate that the smooth terrains were formed by flooding of shallow structural troughs by low-viscosity water-ice lavas. The oldest and most deformed areas (the 'reticulate' terrains) in general have the highest relative elevations, whereas units of the most common resurfaced type--the grooved terrain--lie at elevations between those of the smooth and reticulate terrains. Bright terrain, which accounts for some two-thirds of the surface, probably results from a continuum of processes, including crustal rifting, shallow flooding and groove formation. Volcanism plays an integral role in these processes, and is consistent with partial melting of Ganymede's interior.

Extraterrestrial Environment↗
PubMed2001

Icing Ganymede.

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Ice↗