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Angular momentum dependent friction slows down rotational relaxation under nonequilibrium conditions.

It has recently been shown that relaxation of the rotational energy of hot nonequilibrium photofragments (i) slows down significantly with the increase of their initial rotational temperature and (ii) differs dramatically from the relaxation of the equilibrium rotational energy correlation function, manifesting thereby the breakdown of the linear response description [A. C. Moskun et al., Science 311, 1907 (2006)]. We demonstrate that this phenomenon may be caused by the angular momentum dependence of rotational friction. We have developed the generalized Fokker-Planck equation whose rotational friction depends upon angular momentum algebraically. The calculated rotational correlation functions correspond well to their counterparts obtained via molecular dynamics simulations in a broad range of initial nonequilibrium conditions. It is suggested that the angular momentum dependence of friction should be taken into account while describing rotational relaxation far from equilibrium.

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Microrheometry of semiflexible actin networks through enforced single-filament reptation: frictional coupling and heterogeneities in entangled networks.

Magnetic tweezers are applied to study the enforced motion of single actin filaments in entangled actin networks to gain insight into friction-mediated entanglement in semiflexible macromolecular networks. Magnetic beads are coupled to one chain end of test filaments, which are pulled by 5 to 20 pN force pulses through entangled solutions of nonlabeled actin, the test filaments thus acting as linear force probes of the network. The transient filament motion is analyzed by microfluorescence, and the deflection-versus-time curves of the beads are evaluated in terms of a mechanical equivalent circuit to determine viscoelastic parameters, which are then interpreted in terms of viscoelastic moduli of the network. We demonstrate that the frictional coefficient characterizing the hydrodynamic coupling of the filaments to the surrounding network is much higher than predicted by the tube model, suggesting that friction-mediated interfilament coupling plays an important role in the entanglement of non-cross-linked actin networks. Furthermore, the local tube width along the filament contour (measured in terms of the root-mean-square displacement characterizing the lateral Brownian motion of the test filament) reveals strong fluctuations that can lead to transient local pinching of filaments.

Actin Cytoskeleton↗

Environmental sample correlation with clinical and historical data in a friction product exposure.

Asbestos has been widely used in the past as a component in friction products. A unique setting of dust exposure to such products occurs when individuals are involved with refabrication of the worn components. It is of interest whether asbestos fibers are released from friction materials in the use phase and the postlife phase or if the mineral fibers are converted to a nonasbestos form. In the present study, an individual whose primary work activity had centered on clutch refabrication was evaluated for possible dust-related diseases. Tissue analysis revealed the presence of large numbers of asbestos fibers as well as ferruginous bodies. These particulates were characterized as to composition as well as dimensions. Clutches of the type typically used by this individual were obtained and material was rinsed from their surface for comparative purposes. Materials that were freed from the surface and reviewed by analytical transmission electron microscopy were clearly identifiable as chrysotile asbestos. The composition of the clutch material was compared with the components found in the patient's lung tissue. The conclusion from this comparison was that individuals exposed to friction materials under similar circumstances should use appropriate caution. Appreciable exposure to asbestos can occur and this exposure can be sufficiently high to result in disease.

Air Pollutants, Occupational↗

Friction manipulation for intestinal locomotion.

The importance of colonoscopies on the one hand and the drawbacks of the conventional instrumentation on the other have led to research into alternative colonoscopic devices. The main question for the development of such devices is the method of locomotion along the slippery and flaccid intestinal tube. This paper suggests a new intestinal locomotion method based on friction manipulation between the device and the intestinal wall. A new concept to manipulate friction is described. The concept is based on the active alterations of the friction between the device and the intestinal wall and it is inspired by the locomotion of biological species such as snails and starfish.

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Frictional mechanics of wet granular material.

The mechanical response of a wet granular layer to imposed shear is studied experimentally at low applied normal stress. The granular material is immersed in water and the shear is applied by sliding a plate resting on the upper surface of the layer. We monitor simultaneously the horizontal and the vertical displacements of the plate to submicron accuracy with millisecond time resolution. The relations between the plate displacement, the dilation of the layer and the measured frictional force are analyzed in detail. When slip begins, the dilation increases exponentially over a slip distance comparable to the particle radius. We find that the total dilation and the steady state frictional force do not depend on the driving velocity, but do depend linearly on the applied normal stress. The frictional force also depends linearly on the dilation rate (rather than the dilation itself), and reaches a maximum value during the transient acceleration. We find that the layer can temporarily sustain a shear stress that is in excess of the critical value that will eventually lead to slip. We describe an empirical model that describes much of what we observe. This model differs in some respects from those used previously at stresses 10(6) times larger.

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Shear response of a frictional interface to a normal load modulation

We study the shear response of a sliding multicontact interface submitted to a harmonically modulated normal load, without loss of contact. We measure, at low velocities (V<100 &mgr;m s(-1)), the average value &Fmacr; of the friction force and the amplitude of its first and second harmonic components. The excitation frequency (f=120 Hz) is chosen much larger than the natural one, associated with the dynamical aging of the interface. We show the following: (i) In agreement with the engineering thumb rule, even a modest modulation induces a substantial decrease of &Fmacr;. (ii) The Rice-Ruina state and rate model, though appropriate to describe the slow frictional dynamics, must be extended when dealing with our "high" frequency regime. That is, the rheology which controls the shear strength must explicitly account not only for the plastic response of the adhesive junctions between load-bearing asperities, but also for the elastic contribution of the asperities bodies. This "elastoplastic" friction model leads to predictions in excellent quantitative agreement with all our experimental data.

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Surface stability of granular systems under horizontal and vertical vibration: the applicability of a coefficient of friction

We investigate the conditions under which the surface of a granular pile becomes unstable to vibrations. Three stability boundaries are identified, which depend upon the relative phase of the driving forces and the angle of the prepared slope. The experimental findings can be interpreted within the context of a Coulomb friction model and used to define an effective coefficient of friction. For up-hill motion we find that the coefficient of friction depends strongly on the slope angle and that, in general, it requires less vibration to transport grains uphill than would be otherwise expected.

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Frictional-collisional regime for granular suspension flows down an inclined channel

Here granular suspensions refer to very concentrated suspensions of particles within a Newtonian fluid. Under certain conditions given in the paper, the bulk stresses mainly result from the combination of frictional and collisional interactions at the particle scale. The corresponding flow regime is called the frictional-collisional regime. The constitutive equation adapted to this regime is not well known. We propose a constitutive model based on the balance between frictional and collisional interactions. We have applied this model to granular flow down an inclined channel. It is shown that the mass flow rate is proportional to the flow depth.

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Friction in a solid lubricant film.

Molecular-dynamics study of a thin (one to five layers) lubricant film between two substrates in moving contact are performed using Langevin equations with an external damping coefficient depending on distance and velocity of atoms relative the substrates, motivated by microscopic configurations. They show that the minimal friction coefficient is obtained for the solid-sliding regime. A detailed analysis of the results, the comparison with other microscopic modeling approaches of friction, and the evaluation of quantities that can be compared to experiments, such as the velocity of the transition from stick slip to smooth sliding, are used to discuss the relevance of the microscopic simulations of friction.

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Granular friction, Coulomb failure, and the fluid-solid transition for horizontally shaken granular materials.

We present the results of an extensive series of experiments, molecular dynamics simulations, and models that address horizontal shaking of a layer of granular material. The goal of this work was to better understand the transition between the "fluid" and "solid" states of granular materials. In the experiments, the material-consisting of glass spheres, smooth and rough sand-was contained in a container of rectangular cross section, and subjected to horizontal shaking of the form x=A sin(omega(t)). The base of the container was porous, so that it was possible to reduce the effective weight of the sample by means of a vertical gas flow. The acceleration of the shaking could be precisely controlled by means of an accelerometer mounted onboard the shaker, plus feedback control and lockin detection. The relevant control parameter for this system was the dimensionless acceleration, Gamma=Aomega(2)/g, where g was the acceleration of gravity. As Gamma was varied, the layer underwent a backward bifurcation between a solidlike state that was stationary in the frame of the shaker and a fluidlike state that typically consisted of a sloshing layer of maximum depth H riding on top of a solid layer. That is, with increasing Gamma, the solid state made a transition to the fluid state at Gamma(cu) and once the system was in the fluid state, a decrease in Gamma left the system in the fluidized state until Gamma reached Gamma(cd)<Gamma(cu). In the fluidized state, the flow consisted of back and forth sloshing at the shaker frequency, plus a slower convective flow along the shaking direction and additionally in the horizontal direction transverse to the shaking direction. Molecular dynamics simulations show that the last of these flows is associated with shear and dilation at the vertical sidewalls. For Gamma<Gamma(cu) and in the solid state, there was a "gas" of free particles sliding on the surface of the material. These constituted much less than one layer's worth of particles in all cases. If these "sliders" were suppressed by placing a thin strip of plastic on the surface, the hysteresis was removed, and the transition to fluidization occurred at a slightly lower value than Gamma(cd) for the free surface case. The hysteresis was also suppressed if a vertical gas flow from the base was sufficient to support roughly 40% of the weight of the sample. Both the transition to the fluid state from the solid and the reverse transition from the fluid to the solid were characterized by similar divergent time scales. If Gamma was increased above Gamma(cu) by a fractional amount epsilon=(Gamma-Gamma(cu))/Gamma(cu), where epsilon was small, there was a characteristic time tau=Aepsilon(-beta) for the transition from solid to fluid to occur, where beta is 1.00+/-0.06. Similarly, if Gamma was decreased below Gamma(cd) in the fluidized state by an amount epsilon=(Gamma-Gamma(cd))/Gamma(cd), there was also a transient time tau=Bepsilon(-beta), where beta is again indistinguishable from 1.00. In addition, the amplitudes A and B are essentially identical. By placing a small "impurity" on top of the layer, consisting of a heavier particle, we found that the exponent beta varied as the impurity mass squared and changed by a factor of 3. A simple Coulomb friction model with friction coefficients mu(k)<mu(s) for the fluid and solid states predicts a reversible rather than hysteretic transition to the fluid state, similar to what we observe with the addition of the small overload from a plastic strip. In an improved model, we provide a relaxational mechanism that allows the friction coefficient to change continuously between the low and high values. This model produces the hysteresis seen in experiments.

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Statistics of the contact network in frictional and frictionless granular packings.

Simulated granular packings with different particle friction coefficient mu are examined. The distribution of the particle-particle and particle-wall normal and tangential contact forces P(f) are computed and compared with existing experimental data. Here f identical with F/(-)F is the contact force F normalized by the average value (-)F. P(f) exhibits exponential-like decay at large forces, a plateau/peak near f=1, with additional features at forces smaller than the average that depend on mu. Additional information beyond the one-point force distribution functions is provided in the form of the force-force spatial distribution function and the contact point radial distribution function. These quantities indicate that correlations between forces are only weakly dependent on friction and decay rapidly beyond approximately three particle diameters. Distributions of particle-particle contact angles show that the contact network is not isotropic and only weakly dependent on friction. High force-bearing structures, or force chains, do not play a dominant role in these three-dimensional, unloaded packings.

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Friction effects and clogging in a cellular automaton model for pedestrian dynamics.

We investigate the role of conflicts in pedestrian traffic, i.e., situations where two or more people try to enter the same space. Therefore a recently introduced cellular automaton model for pedestrian dynamics is extended by a friction parameter mu. This parameter controls the probability that the movement of all particles involved in a conflict is denied at one time step. It is shown that these conflicts are not an undesirable artifact of the parallel update scheme, but are important for a correct description of the dynamics. The friction parameter mu can be interpreted as a kind of an internal local pressure between the pedestrians which becomes important in regions of high density, occurring, e.g., in panic situations. We present simulations of the evacuation of a large room with one door. It is found that friction has not only quantitative effects, but can also lead to qualitative changes, e.g., of the dependence of the evacuation time on the system parameters. We also observe similarities to the flow of granular materials, e.g., arching effects.

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Quasi-two-dimensional turbulence in shallow fluid layers: the role of bottom friction and fluid layer depth.

The role of bottom friction and the fluid layer depth in numerical simulations and experiments of freely decaying quasi-two-dimensional turbulence in shallow fluid layers has been investigated. In particular, the power-law behavior of the compensated kinetic energy E0(t)=E(t)e(2lambda t), with E(t) the total kinetic energy of the flow and lambda the bottom-drag coefficient, and the compensated enstrophy Omega(0)(t)=Omega(t)e(2lambda t), with Omega(t) the total enstrophy of the flow, have been studied. We also report on the scaling exponents of the ratio Omega(t)/E(t), which is considered as a measure of the characteristic length scale in the flow, for different values of lambda. The numerical simulations on square bounded domains with no-slip boundaries revealed bottom-friction independent power-law exponents for E0(t), Omega(0)(t), and Omega(t)/E(t). By applying a discrete wavelet packet transform technique to the numerical data, we have been able to compute the power-law exponents of the average number density of vortices rho(t), the average vortex radius a(t), the mean vortex separation r(t), and the averaged normalized vorticity extremum omega(ext)(t)/square root E(t). These decay exponents proved to be independent of the bottom friction as well. In the experiments we have varied the fluid layer depth, and it was found that the decay exponents of E0(t), Omega(0)(t), Omega(t)/E(t), and omega(ext)(t)/square root E(t) are virtually independent of the fluid layer depth. The experimental data for rho(t) and a(t) are less conclusive; power-law exponents obtained for small fluid layer depths agree with those from previously reported experiments, but significantly larger power-law exponents are found for experiments with larger fluid layer depths.

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Kinetic friction and atomistic instabilities in boundary-lubricated systems.

The contribution of sliding-induced, atomic-scale instabilities to the kinetic friction force is investigated by molecular dynamics. For this purpose, we derive a relationship between the kinetic friction force F(k) and the nonequilibrium velocity distribution P(v) of the lubricant particles. P(v) typically shows exponential tails, which cannot be described in terms of an effective temperature. It is investigated which parameters control the existence of instabilities and how they affect P(v) and hence F(k). The effects of the interfaces' dimensionality, lubricant coverage, and internal degrees of freedom of lubricant particles on F(k) are studied explicitly. Among other results, we find that the kinetic friction between commensurate surfaces is much more susceptible to changes in (i) lubricant coverage, (ii) sliding velocity, and (iii) bond length of lubricant molecules than incommensurate surfaces.

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Onset of incommensurate interfacial instability in a minimal model of dry friction.

We present a minimal model of dry friction between two incommensurate interfaces sliding at high relative velocity. Many of the features of the friction force for the full two-dimensional many-body dynamical system-particularly in the sub-critical velocity regime-are captured by our one-dimensional Einstein model, where the motion of a typical interfacial atom is constrained to be vertical to the sliding plane. Beyond the linear response of force versus sliding velocity, the anharmonic Einstein model predicts a doublet resonance peak, whereupon a catastrophe in the model signals the onset of a plastic deformation mechanism for frictional sliding, namely, the instability of the interface. Higher velocities than this critical value require a much more sophisticated description of the production and coalescence of dislocations into a microstructure.

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Friction measurements in granular media.

We present some experimental results, estimating the lateral stress response to a longitudinal stress applied to an ideal granular system as a function of friction parameters. Structural effects are taken into account through the use of an angle of contact distribution. The two-dimensional model, based on mainly equally sized cylinder granules allows one to derive a dependency of the friction between single granules and the overall angle of friction, which is commonly used to describe the macroscopic behavior of granulate material.

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Thermally induced suppression of friction at the atomic scale.

Atomic-scale friction, as accessed in tip-based experiments, is investigated theoretically in the full range of surface corrugations, temperatures, and velocities. Emphasis is given to the regime of thermal drift, when the regular stick-slip behavior is completely ruined by thermal effects. The possibility of nearly vanishing friction ("thermolubricity") is predicted even for strong (overcritical) surface corrugations, when traditional models would predict significant friction. The manifestation of this effect in recently published experimental data is demonstrated.

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Friction of -bead macromolecules in solution: effects of the bead-solvent interaction.

The role of the bead-solvent interaction has been studied for its influence on the dynamics of an N-bead macromolecule which is immersed into a solution. Using a Fokker-Planck equation for the phase-space distribution function of the macromolecule, we show that all the effects of the solution can be treated entirely in terms of the friction tensors which are assigned to each pair of interacting beads in the chain. For the high-density as well as for the critical solvent, the properties of these tensors are discussed in detail and are calculated by using several (realistic) choices of the bead-solvent potential. From the friction tensors, moreover, an expression for the center-of-mass friction coefficient of a (N-bead) chain macromolecule is derived. Numerical data for this coefficient for "truncated" Lennard-Jones bead-solvent potential are compared with results from molecular dynamic simulations and from the phenomenological theoretical data as found in the literature.

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