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PubMed2004

Radon in well waters in the Kraków area.

The method and the results of radon concentration measurements in water samples are presented. Since May 2000, measurements of radon concentration in well waters in the Kraków area have been carried out--both in urban wells (depth above 50 meters) and in other private wells (depth of several meters). The ionisation chamber AlphaGUARD PQ 2000PRO along with the additional special equipment AquaKIT were used for determination of radon concentration in water samples. A total of 45 wells were examined for radon concentration in water--19 urban wells, 21 private ones (from Nowa Huta, Ojcowska, Wola Justowska area--parts of Kraków) and 5 mineral water sources. Wola Justowska is a region where tectonics faults occur and radon can easily migrate from deep basement structure. All the obtained values of radon concentration are below 12 Bq/l. These preliminary results do not show a direct correlation between geological structure and radon concentration in water samples. However, further investigation is needed and is planned to be undertaken.

Environmental Monitoring↗
PubMed2006

Correlation test between indoor radon and surficial gamma radiation in Northern Virginia.

In northern Virginia, significant indoor radon differences occur due to soil chemistry, home heating system and precipitation. Homes constructed on soil over some geological units had indoor radon that exceeded the United States Environmental Protection Agency Maximum Concentration Level of 4 picoCuries/liter for home buyers. Seasons with more precipitation tend to have higher average indoor radon. Homes with electrical heating systems averaged almost 50% higher indoor radon than homes with gas or oil furnaces. Comparisons between indoor radon and soil radon show a positive correlation, suggesting that soil aero radioactivity measurements can delineate areas with a high potential for indoor radon.

Air Pollutants, Radioactive↗
PubMed2006

Impact of measurement error in exposures in german radon studies.

Case-control studies on lung cancer and residential radon exposure were conducted in West and East Germany. Odds ratio (OR) estimates from primary analysis are now subject to correction for measurement error in exposure. We apply the regression calibration method adopting a bivariate multiplicative error model of the classical type; that is, we investigate the impact of errors in the exposure of primary interest, radon, and of errors in the most potent confounder, smoking. The OR estimates per 100 Bq/m3 are throughout higher after correcting for errors in radon exposure (e.g., 1.02 and 1.11 for the West and the East German study, respectively, corrected for an error of size 0.4); ignoring the clear but small correlation between radon exposure and smoking of about -0.06 would lead to less conservative corrections (1.10 and 1.13 for West and East, respectively). Accounting for a realistically sized error in the smoking variable additionally increases the OR estimates slightly. Remarkable is the fact that the naive OR estimate of the West study of 0.97 exceeds unity after correcting for errors in radon exposure larger than 0.3. We conclude that correcting for errors in radon exposure has a meaningful impact on OR estimates, that the correlation between radon exposure and the smoking variable affects the correction even if the smoking variable was error-free, and that such an analysis is extremely valuable to grasp an important issue in epidemiology, that is, the dimension of residual confounding due to adjusting for an imprecisely measured smoking variable.

Air Pollutants, Radioactive↗
PubMed2001

Variations of well water radon in Virginia and Maryland.

In north-central Virginia and south-central Maryland, municipal water supplies obtained from reservoirs provide radon-free potable water. However, about 10 percent of the population consumes well water. Radon in drinking water from some wells exceeds 4,000 pCi/L. Only about 30% of the radon is lost between the well storage tanks and the homes. The average radon concentration is about 2,000 pCi/L, which greatly exceeds the U.S. Environmental Protection Agency's recommended Maximum Contamination Level of 300 pCi/L. In this study of a geologically diverse area, the well water comes from granite (radon averages about 3,000 pCi,/L), schist and phyllite (about 2,000 pCi/L), sandstone (about 1,500 pCi/L), and quartzite (about 1,100 pCi/L). Aeration experiments on well water in storage tanks indicated that about 60-70% can be removed using a splash box with an exhaust fan on the storage tank, and about 60-70% can be removed using bubble aeration. About 90% of the radon can be removed by the simultaneous use of bubble aeration, splash box, and an exhaust fan. However, this combination does not become less efficient through time. Passing the water through tanks of activated charcoal can remove about 90% of the radon, though the charcoal becomes less efficient over an interval of a few months.

Air↗
PubMed2003

Radon concentration in Jordanian drinking water and hot springs.

The radon concentration in Jordanian drinking water and hot springs has been measured using the electret-passive environmental radon monitoring method. This study maps out Jordanian water sources from the north to the south as well as the area around the capital Amman and the Jordan valley. Samples from 30 sources were collected and analysed during the period from November 2001 to June 2002. We have found that 60% of the drinking water sources have radon concentrations above the proposed US Environmental Protection Agency limit of 11 Bq l(-1); these are mostly situated in the northern region of the country. Fortunately, these sources supplied only a small number of people since they were mainly located in rural areas. Tap water in the capital Amman, where approximately 35% of the population live, has a very low radon concentration, 3.9 Bq l(-1). However, the isolated northern drinking water wells did show a radon level as high as 117 Bq l(-1). Hot springs in Jordan have a radon level ranging between 63 and 81 Bq l(-1), again mainly in the northern region. In general we conclude that Jordanian drinking water is safe as far as radon concentration is concerned with the exception of a few isolated local drinking water wells.

Environmental Monitoring↗
PubMed1995

Radon and cancers other than lung cancer in underground miners: a collaborative analysis of 11 studies.

BACKGROUND: Exposure to the radioactive gas radon and its progeny (222Rn and its radioactive decay products) has recently been linked to a variety of cancers other than lung cancer in geographic correlation studies of domestic radon exposure and in individual cohorts of occupationally exposed miners. PURPOSE: This study was designed to characterize further the risks for cancers other than lung cancer (i.e., non-lung cancers) from atmospheric radon. METHODS: Mortality from non-lung cancer was examined in a collaborative analysis of data from 11 cohorts of underground miners in which radon-related excesses of lung cancer had been established. The study included 64,209 men who were employed in the mines for 6.4 years on average, received average cumulative exposures of 155 working-level months (WLM), and were followed for 16.9 years on average. RESULTS: For all non-lung cancers combined, mortality was close to that expected from mortality rates in the areas surrounding the mines (ratio of observed to expected deaths [O/E] = 1.01; 95% confidence interval [CI] = 0.95-1.07, based on 1179 deaths), and mortality did not increase with increasing cumulative exposure. Among 28 individual cancer categories, statistically significant increases in mortality for cancers of the stomach (O/E = 1.33; 95% CI = 1.16-1.52) and liver (O/E = 1.73; 95% CI = 1.29-2.28) and statistically significant decreases for cancers of the tongue and mouth (O/E = 0.52; 95% CI = 0.26-0.93), pharynx (O/E = 0.35; 95% CI = 0.16-0.66), and colon (O/E = 0.77; 95% CI = 0.63-0.95) were observed. For leukemia, mortality was increased in the period less than 10 years since starting work (O/E = 1.93; 95% CI = 1.19-2.95) but not subsequently. For none of these diseases was mortality significantly related to cumulative exposure. Among the remaining individual categories of non-lung cancer, mortality was related to cumulative exposure only for cancer of the pancreas (excess relative risk per WLM = 0.07%; 95% CI = 0.01-0.12) and, in the period less than 10 years since the start of employment, for other and unspecified cancers (excess relative risk per WLM = 0.22%; 95% CI = 0.08-0.37). CONCLUSIONS: The increases in mortality from stomach and liver cancers and leukemia are unlikely to have been caused by radon, since they are unrelated to cumulative exposure. The association between cumulative exposure and pancreatic cancer seems likely to be a chance finding, while the association between cumulative exposure and other and unspecified cancers was caused by deaths certified as due to carcinomatosis (widespread disseminated cancer throughout the body) that were likely to have been due to lung cancers. This study, therefore, provides considerable evidence that high concentrations of radon in air do not cause a material risk of mortality from cancers other than lung cancer. IMPLICATIONS: Protection standards for radon should continue to be based on consideration of the lung cancer risk alone.

Adult↗
PubMed1994

Assessment of ecologic regression in the study of lung cancer and indoor radon.

Ecologic regression studies conducted to assess the cancer risk of indoor radon to the general population are subject to methodological limitations, and they have given seemingly contradictory results. The authors use simulations to examine the effects of two major methodological problems that affect these studies: measurement error and misspecification of the risk model. In a simulation study of the effect of measurement error caused by the sampling process used to estimate radon exposure for a geographic unit, both the effect of radon and the standard error of the effect estimate were underestimated, with greater bias for smaller sample sizes. In another simulation study, which addressed the consequences of uncontrolled confounding by cigarette smoking, even small negative correlations between county geometric mean annual radon exposure and the proportion of smokers resulted in negative average estimates of the radon effect. A third study considered consequences of using simple linear ecologic models when the true underlying model relation between lung cancer and radon exposure is nonlinear. These examples quantify potential biases and demonstrate the limitations of estimating risks from ecologic studies of lung cancer and indoor radon.

Bias↗
PubMed2003

Seasonal correction factors for estimating radon exposure in dwellings in France.

Indoor radon concentrations are subject to seasonal variation with a maximum in winter and a minimum in summer. Procedures to correct for seasonal variation are necessary in order to get an unbiased estimate of the annual average radon concentration from data based on short-period radon measurements. To obtain correction factors, we apply the model developed by Pinel et al to the French database of indoor radon measurements (measurements performed as part of the indoor radon case-control study and of the national radon measurement campaign). For 6-month measurements, the correction factors vary from 0.87 to 1.17 and agree with those previously published. These results might be applicable when assessing indoor radon concentrations with regard to recommended action levels.

Air Pollutants, Radioactive↗
PubMed2003

Characterisation of an electronic radon gas personal dosemeter.

The monitoring of radon exposure at workplaces is of great importance. Up to now passive measurement systems have been used for the registration of radon gas. Recently an electronic radon gas personal dosemeter came onto the market as an active measurement system for the registration of radon exposure (DOSEman; Sarad GmbH, Dresden, Germany). In this personal monitor, the radon gas diffuses through a membrane into a measurement chamber. A silicon detector system records spectroscopically the alpha decays of the radon gas and of the short-lived progeny 218Po and 214Po gathered onto the detector by an electrical field. In this work the calibration was tested and a proficiency test of this equipment was made. The diffusion behaviour of the radon gas into the measurement chamber, susceptibility to thoron, efficiency, influence of humidity, accuracy and the detection limit were checked.

Air Pollutants, Radioactive↗
PubMed2001

Radon survey in Kalamata (Greece).

A national radon survey is still lacking for Greece. Some groups have carried out several more or less local or extended radon surveys and valuable experience has been gained. After the first preliminary survey carried out by our group, where 500 Kodak LR-115 etched track detectors were placed in Greek schools and dwellings for one year, indoor radon measurements were continued by placing the same number of detectors in a restricted area, covering the city of Kalamata (a medium size city with 60,000 inhabitants), situated in the south of Peloponnese. Although Kalamata was not of special radon interest, the local authorities insisted on knowing for their citizens' sake the level of this natural radiation. At first, the intention was to use a different method of organisation and distribution of the etched-track detectors from the previous one, attempting mainly to acquire more reliable results and to collect as many detectors as possible. Secondly, it was of great importance to test the statistics of the indoor radon concentrations for a rather small area, and thirdly, to estimate independently the annual absorbed dose by children, taking into account radon concentrations measured both in their home and at school. The set of detectors' readings (about 370), revealed, in general, lower values for Kalamata, compared to the ones found in the preliminary radon survey in Greece and almost all concentrations were found to be below the NRPB action level (200 Bq.m-3).

Air Pollution, Indoor↗
PubMed2004

Theory of radon exhalation into accumulators placed at the soil-atmosphere interface.

A theoretical analysis is provided for the phenomenon of radon diffusion into cylindrical accumulators (inverted cups), which are commonly used for the measurement of radon exhalation rates from the earth's surface. Analytical solutions to the diffusion equations in the soil and the cup spaces are obtained by a two-dimensional (2-D) analysis that takes into account the perturbation in the horizontal and vertical radon concentration profiles brought about by the presence of the cup. The mixed nature of the boundary conditions at the soil surface and the cup-soil interface is handled by dual integral equation techniques. The treatment includes steady-state and time-dependent situations with and without ventilation. Formulae are derived for the effective time constant of radon build-up in the cup and for the back diffusion correction factors in different experimental situations. It is found that the effective time constant of radon build-up is much larger than the radon decay constant and it increases for smaller cups. The back diffusion correction factors to be employed in one-time measurement methods also increase as the cup dimensions decrease. The present work provides an analytical basis of an earlier numerical treatment for the growth curve analysis of the same problem. Although the results are based on the assumptions of somewhat ideal nature for mathematical tractability, they provide upper bound estimates of the phenomenon of back diffusion. Some practical applications of the results for extracting diffusion length of radon in materials are also suggested.

Atmosphere↗
PubMed2005

Development of a radon trap device using a corona discharge.

Radon is one of the noble gases, which are chemically inert and do not make any reactants under normal conditions. In this experiment we demonstrated an enigmatic reaction between radon and fluorine when a corona discharge is used as a promoter. Distinctive changes in radon concentrations were caused by the discharge and a trap efficiency of >99.5% was estimated. The mass balance between the trapped and the released radon was found to be reasonable. This indicates the existence of chemical reactions with radon. This trap phenomenon has application as a technique for reducing radon concentration in radon-contaminated air. It is possible that this technique will be applicable to other noble gases.

Air Pollutants, Radioactive↗
PubMed2006

Indoor radon concentration in the rural dwellings of Chhattisgarh state (India).

Inhalation of radon and its daughter products is the major contributor to the total exposure of the population to natural radiation. An indoor radon survey has been carried out in the state of Chhattisgarh (80.26 degrees N to 84.41 degrees N and 17.8 degrees E to 24.1 degrees E), India under the national coordinated radon project of the Department of Atomic Energy. In the frame of this project indoor radon concentration has been measured in 105 dwellings situated in different villages of Chhattisgarh state. Houses were selected for measurements to cover the most common type of houses generally existing in the rural areas. Measurements have been done on quarterly integrating cycle for one full year in each dwelling using radon cup dosemeter employing LR-115, type-II (pelliculable), solid-state nuclear track detectors. The gamma radiation level was also checked in each dwelling using a gamma survey meter. It was found that the annual average indoor radon concentration in these dwellings varies from 9.91 to 87.84 Bq m(-3) with overall mean value of 26.48 Bq m(-3). Gamma level in these rural dwellings varies from 14.84 to 26.56 microR h(-1) with mean value of 18.68 microR h(-1). We observed that the radon concentration is relatively higher in the houses where the floor is bare but relatively lower in those houses where the floor is tiled or cemented.

Air Pollution, Indoor↗
PubMed1990

Predicted reduction in lung cancer risk following cessation of smoking and radon exposure.

Recently there has been considerable public and regulatory concern that radon, produced by the decay of naturally occurring uranium, can accumulate in homes, offices, and schools at levels that may substantially increase the risk of lung cancer. The major cause of lung cancer is smoking, and radon appears to interact multiplicatively with smoking in causing lung cancer. Thus, the most effective way to reduce the increased risk of lung cancer resulting from radon exposure is to cease smoking. In this paper, a model for the risks associated with radon exposure that was developed by a committee of the National Academy of Sciences is used to calculate the benefits, in terms of reduction in lifetime risk of lung cancer, of ceasing to smoke, ceasing radon exposure, or ceasing both. Ceasing to smoke is considerably more beneficial than ceasing radon exposure, and thus policymakers addressing the health effects of radon should place priority on encouraging individuals to stop smoking.

Adult↗
PubMed1984

Passive, integrated measurement of indoor radon using activated carbon.

Activated carbon canisters were tested to determine their adsorption and retention characteristics for radon. Our tests conducted indoors under typical conditions of temperature and relative humidity indicate that simple, inexpensive and maintenance-free passive devices containing 150-200 g of activated carbon can measure radon conveniently and adequately. The amount of radon absorbed in the collector is determined by counting the gamma rays from the decay products of radon. The lower limit of detection for radon is 0.2 pCi/l. for an exposure of 72 hr. Greater sensitivity can be obtained with larger counting systems and devices containing carbon with more surface area. Tests in a residential building and in a test chamber indicate that the measured radon in the canister is proportional to the mean concentration of radon during the period of exposure when correction for relative humidity is made. For practical situations encountered indoors, the device yields results accurate to within +/- 20%. Results from field measurements indicate that the use of the device is feasible.

Air Pollutants↗
PubMed1993

Modeling radon entry into Florida slab-on-grade houses.

Radon entry into a Florida house whose concrete slab is supported by a permeable concrete-block stem wall and a concrete footer is modeled. The slab rests on backfill material; the same material is used to fill the footer trench. A region of undisturbed soil is assumed to extend 10 m beyond and below the footer. The soil is assumed homogeneous and isotropic except for certain simulations in which soil layers of high permeability or radium content are introduced. Depressurization of the house induces a pressure field in the soil and backfill. The Laplace equation, resulting from Darcy's law and the continuity equation, is solved using a steady-state finite-difference model to determine this field. The mass-transport equation is then solved to obtain the diffusive and advective radon entry rates through the slab; the permeable stem wall; gaps at the intersections of the slab, stem wall, and footer; and gaps in the slab. These rates are determined for variable soil, backfill, and stem-wall permeability and radium content, slab-opening width and position, slab and stem-wall diffusivity, and water table depth. The variations in soil permeability and radium content include cases of horizontally stratified soil. We also consider the effect of a gap between the edge of the slab and the stem wall that restricts the passage of soil gas from the stem wall into the house. Calculations indicate that the total radon entry rate is relatively low unless the soil or backfill permeability or radium content is high. Variations in most of the factors, other than the soil permeability and radium content, have only a small effect on the total radon entry rate. However, for a fixed soil permeability, the total radon entry rate may be reduced by a factor of 2 or more by decreasing the backfill permeability, by making the stem wall impermeable and gap-free, (possibly by constructing a one-piece slab/stem-wall/footer), or by increasing the pressure in the interior of the stem wall (by ensuring that there is a large pressure drop across the slab/stem-wall gap), thereby reducing radon entry into the wall from the soil. Use of an impermeable stem wall and a low-permeability fill in combination is predicted to reduce the radon entry rate by 71%.

Air Pollution, Indoor↗
PubMed1994

Influence of ventilation strategies on indoor radon concentrations based on a semiempirical model for Florida-style houses.

Measurements in a full-scale experimental facility are used to benchmark a semiempirical model for predicting indoor radon concentrations for Florida-style houses built using slab-on-grade construction. The model is developed to provide time-averaged indoor radon concentrations from quantitative relationships between the time-dependent radon entry and elimination mechanisms that have been demonstrated to be important for this style of residential construction. The model successfully predicts indoor radon concentrations in the research structure for several pressure and ventilation conditions. Parametric studies using the model illustrate how different ventilation strategies affect indoor radon concentrations. It is demonstrated that increasing house ventilation rates by increasing the effective leakage area of the house shell does not reduce indoor radon concentrations as effectively as increasing house ventilation rates by controlled duct ventilation associated with the heating, ventilating, and air conditioning system. The latter strategy provides the potential to minimize indoor radon concentrations while providing positive control over the quality of infiltration air.

Air Pollution, Indoor↗
PubMed1994

The effect of aging, humidity, and fly-ash additive on the radon exhalation from concrete.

Radon exhalation rates of concrete samples have been periodically determined for 6-8 y after pouring the concrete. From the results, it can be concluded that the radon exhalation rate changes with the age of the concrete. The exhalation rate varies considerably in the first 6-12 mo after pouring with a factor of 1.5. After this period, the variation in exhalation rates is much less. Starting 1 y after pouring, the radon exhalation rate was decreased with increasing age of concrete to 0.3-0.6 of the maximum at the end of the observed period. Low humidity conditions dramatically reduce the radon exhalation rate of concrete. If 25% by volume of the cement is replaced by fly ash, the 226Ra concentration is elevated by a factor of 1.5. The radon exhalation rate of concrete made with Portland cement and fly ash was increased only slightly or even decreased, despite the higher 226Ra content. The results indicate that measurements of radon exhalation from samples of concrete have to be standardized on a certain humidity and age of the sample. Under certain conditions, the addition of fly ash to the concrete can reduce the radon exhalation.

Air Pollutants, Radioactive↗