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PubMed2002

Identification of iron sulphide grains in protoplanetary disks.

Sulphur is depleted in cold dense molecular clouds with embedded young stellar objects, indicating that most of it probably resides in solid grains. Iron sulphide grains are the main sulphur species in cometary dust particles, but there has been no direct evidence for FeS in astronomical sources, which poses a considerable problem, because sulphur is a cosmically abundant element. Here we report laboratory infrared spectra of FeS grains from primitive meteorites, as well as from pyrrhotite ([Fe, Ni](1-x)S) grains in interplanetary dust, which show a broad FeS feature centred at approximately 23.5 micrometres. A similar broad feature is seen in the infrared spectra of young stellar objects, implying that FeS grains are an important but previously unrecognized component of circumstellar dust. The feature had previously been attributed to FeO. The observed astronomical line strengths are generally consistent with the depletion of sulphur from the gas phase, and with the average Galactic sulphur/silicon abundance ratio. We conclude that the missing sulphur has been found.

Journal Article↗
PubMed1987

Comets and life.

Some of the chemical species which have been detected in comets include H2O, HCN, CH3CN, CO, CO2, NH3, CS, C2 and C3. All of these have also been detected in the interstellar medium, indicating a probable relationship between interstellar dust and gas clouds and comets. Laboratory experiments carried out with different mixtures of these molecules give rise to the formation of the biochemical compounds which are necessary for life, such as amino acids, purines, pyrimidines, monosaccharides, etc. However, in spite of suggestions to the contrary, the presence of life in comets is unlikely. On the other hand, the capture of cometary matter by the primitive Earth is considered essential for the development of life on this planet. The amount of cometary carbon-containing matter captured by the Earth, as calculated by different authors, is several times larger than the total amount of organic matter present in the biosphere (10(18)g). The major classes of reactions which were probably involved in the formation of key biochemical compounds are discussed. Our tentative conclusions are that: 1) comets played a predominant role in the emergence of life on our planet, and 2) they are the cosmic connection with extraterrestrial life.

Atmosphere↗
PubMed1999

Cross-Correlation of Tenerife Data with Galactic Templates-Evidence for Spinning Dust?

The recent discovery of dust-correlated diffuse microwave emission has prompted two rival explanations: free-free emission and spinning dust grains. We present new detections of this component at 10 and 15 GHz by the switched-beam Tenerife experiment. The data show a turnover in the spectrum and thereby support the spinning dust hypothesis. We also present a significant detection of synchrotron radiation at 10 GHz, which is useful for normalizing foreground contamination of cosmic microwave background experiments at high galactic latitudes.

Journal Article↗
PubMedDate not supplied

Critical issues in connection with human planetary missions: protection of and from the environment.

Activities associated with human missions to the Moon or to Mars will interact with the environment in two reciprocal ways: (i) the mission needs to be protected from the natural environmental elements that can be harmful to human health, the equipment or to their operations: (ii) the specific natural environment of the Moon or Mars should be protected so that it retains its value for scientific and other purposes. The following environmental elements need to be considered in order to protect humans and the equipment on the planetary surface: (i) cosmic ionizing radiation, (ii) solar particle events; (iii) solar ultraviolet radiation; (iv) reduced gravity; (v) thin atmosphere; (vi) extremes in temperatures and their fluctuations; (vii) surface dust; (viii) impacts by meteorites and micrometeorites. In order to protect the planetary environment. the requirements for planetary protection as adopted by COSPAR for lander missions need to be revised in view of human presence on the planet. Landers carrying equipment for exobiological investigations require special consideration to reduce contamination by terrestrial microorganisms and organic matter to the Greatest feasible extent. Records of human activities on the planet's surface should be maintained in sufficient detail that future scientific experimenters can determine whether environmental modifications have resulted from explorations. Grant numbers: 14056/99/NL/PA.

Aerospace Medicine↗
PubMed2003

Critical issues in connection with human missions to Mars: protection of and from the Martian environment.

Human missions to Mars are planned to happen within this century. Activities associated therewith will interact with the environment of Mars in two reciprocal ways: (i) the mission needs to be protected from the natural environmental elements that can be harmful to human health, the equipment or to their operations; (ii) the specific natural environment of Mars should be protected so that it retains its value for scientific and other purposes. The following environmental elements need to be considered in order to protect humans and the equipment on the planetary surface: (i) cosmic ionizing radiation, (ii) solar particle events; (iii) solar ultraviolet radiation; (iv) reduced gravity; (v) thin atmosphere; (vi) extremes in temperatures and their fluctuations; and (vii) surface dust. In order to protect the planetary environment, the requirements for planetary protection as adopted by COSPAR for lander missions need to be revised in view of human presence on the planet. Landers carrying equipment for exobiological investigations require special consideration to reduce contamination by terrestrial microorganisms and organic matter to the greatest feasible extent. Records of human activities on the planet's surface should be maintained in sufficient detail that future scientific experimenters can determine whether environmental modifications have resulted from explorations.

Aerospace Medicine↗
PubMed2005

The obscuration by dust of most of the growth of supermassive black holes.

Supermassive black holes underwent periods of exponential growth during which we see them as quasars in the distant Universe. The summed emission from these quasars generates the cosmic X-ray background, the spectrum of which has been used to argue that most black-hole growth is obscured. There are clear examples of obscured black-hole growth in the form of 'type-2' quasars, but their numbers are fewer than expected from modelling of the X-ray background. Here we report the direct detection of a population of distant type-2 quasars, which is at least comparable in size to the well-known unobscured type-1 population. We selected objects that have mid-infrared and radio emissions characteristic of quasars, but which are faint at near-infrared and optical wavelengths. We conclude that this population is responsible for most of the black-hole growth in the young Universe and that, throughout cosmic history, black-hole growth occurs in the dusty, gas-rich centres of active galaxies.

Journal Article↗
PubMed1995

The interstellar carbon budget and the role of carbon in dust and large molecules.

Published data on stellar composition show that carbon in the sun is substantially more abundant than in other stars. A carbon abundance of 225 carbon atoms per 10(6) hydrogen atoms is representative of galactic stars, whereas published values for the sun range from 350 to 470 carbon atoms per 10(6) hydrogen atoms. Other elements are also present in enhanced quantities in the solar system, consistent with suggestions that a supernova event was closely associated with the formation of the solar system. The overabundance of carbon in the solar system has many important implications, including new constraints on nucleosynthesis models for supernovae and substantial modification of the so-called "cosmic" composition normally adopted in discussions of galactic and interstellar abundances. A reduction in the galactic carbon budget, as suggested by the stellar composition data, strongly constrains the quantity of carbon that is available for the formation of interstellar dust, and some dust models now appear implausible because they require more carbon than is available.

Carbon↗
PubMed1996

Extraterrestrial helium trapped in fullerenes in the Sudbury impact structure.

Fullerenes (C60 and C70) in the Sudbury impact structure contain trapped helium with a 3He/4He ratio of 5.5 x 10(-4) to 5.9 x 10(-4). The 3He/4He ratio exceeds the accepted solar wind value by 20 to 30 percent and is higher by an order of magnitude than the maximum reported mantle value. Terrestrial nuclear reactions or cosmic-ray bombardment are not sufficient to generate such a high ratio. The 3He/4He ratios in the Sudbury fullerenes are similar to those found in meteorites and in some interplanetary dust particles. The implication is that the helium within the C60 molecules at Sudbury is of extraterrestrial origin.

Carbon↗
PubMed1992

Infrared spectroscopy of dense clouds in the C-H stretch region: methanol and "diamonds."

High spectral resolution (nu/delta nu = 900) studies in the 3100-2600 cm-1 (3.2-3.9 microns) range are presented of the protostars NGC 7538 IRS 9, W33A, W3 IRS 5, and S140 IRS 1. This is the spectral region in which the fundamental C-H stretching vibrations of aliphatic hydrocarbons fall. Well-resolved absorption bands at about 2825 cm-1 (3.54 microns) and 2880 cm-1 (3.47 microns) were found superposed on the low-frequency wing of the strong O-H stretch feature. The 2880 cm-1 (3.47 microns) band, a new interstellar feature, is moderately strong in the spectra of all four objects studied. The 2825 cm-1 (3.54 microns) band, previously detected toward W33A, is also in the spectrum of NGC 7538 IRS 9. The relative strength of these two bands varies, showing that they are associated with two different carriers. On the basis of comparisons with laboratory spectra, the 2825 cm-1 (3.54 microns) band is assigned to methanol (CH3OH), in agreement with the earlier work of Grim et al. (1991). This assignment is further supported by a pair of weak absorptions centered at 2600 and 2540 cm-1 (3.85 and 3.94 microns) in the spectrum of W33A recently reported by Geballe (1991). These features compare very well with laboratory spectra of CH3OH/H2O ice mixtures. The CH3OH/H2O ratio derived from the 2825 cm-1 methanol band and the 3250 cm-1 (3.08 microns) H2O feature are 0.13 and 0.40 for NGC 7538 IRS 9 and W33A, respectively. These values are smaller than the ratios of 0.61 and 0.54 derived using the 1460 cm-1 (6.85 microns) band assigned to CH3OH and the 1665 cm-1 (6.00 microns) H2O band. These apparent discrepancies may be due to a combination of scattering effects within the molecular cloud, uncertainties associated with the baselines for the 2825 cm-1 feature, and the presence of other interstellar grain materials that absorb at 1460 cm-1 (6.85 microns). Nonetheless, after H2O, CH3OH is the most abundant known interstellar ice constituent. The new band at about 2880 cm-1 (3.47 microns) falls near the position for C-H stretching vibrations in tertiary carbon atoms. The strength of this feature, in combination with the lack of strong features associated with primary (-CH3) and secondary (-CH2-) carbon atoms, suggests that the carrier of the new feature has a diamond-like structure. We therefore tentatively attribute this new feature to interstellar "diamonds." The detection of this band in the spectra of all four dense molecular clouds suggests that the carrier is ubiquitous in dense clouds. Band-strength analysis indicates that a minimum of a few percent of the available cosmic carbon is tied up in this material.

Astronomical Phenomena↗
PubMed2004

The annual effective dose from natural sources of ionising radiation in Canada.

A review and analysis of published information combined with the results of recent gamma ray surveys were used to determine the annual effective dose to Canadians from natural sources of radiation. The dose due to external radiation was determined from ground gamma ray surveys carried out in the cities of Toronto, Ottawa, Montreal and Winnipeg and was calculated to be 219 microSv. A compilation of airborne gamma ray data from Canada and the United States shows that there are large variations in external radiation with the highest annual outdoor level of 1424 microSv being found in northern Canada. The annual effective inhalation dose of 926 microSv from 222Rn and 220Rn was calculated from approximately 14,000 measurements across Canada. This value includes a contribution of 128 microSv from 222Rn in the outdoor air together with 6 microSv from long-lived uranium and thorium series radionuclides in dust particles. Based on published information, the annual effective dose due to internal radioactivity is 306 microSv. A program developed by the Federal Aviation Administration was used to calculate a population-weighted annual effective dose from cosmic radiation of 318 microSv. The total population-weighted average annual effective dose to Canadians from all sources of natural background radiation was calculated to be 1769 microSv but varies significantly from city to city, largely due to differences in the inhalation dose from 222Rn.

Background Radiation↗
PubMed1997

Detection of organic matter in interstellar grains.

Star formation and the subsequent evolution of planetary systems occurs in dense molecular clouds, which are comprised, in part, of interstellar dust grains gathered from the diffuse interstellar medium (DISM). Radio observations of the interstellar medium reveal the presence of organic molecules in the gas phase and infrared observational studies provide details concerning the solid-state features in dust grains. In particular, a series of absorption bands have been observed near 3.4 microns (approximately 2940 cm-1) towards bright infrared objects which are seen through large column densities of interstellar dust. Comparisons of organic residues, produced under a variety of laboratory conditions, to the diffuse interstellar medium observations have shown that aliphatic hydrocarbon grains are responsible for the spectral absorption features observed near 3.4 microns (approximately 2940 cm-1). These hydrocarbons appear to carry the -CH2- and -CH3 functional groups in the abundance ratio CH2/CH3 approximately 2.5, and the amount of carbon tied up in this component is greater than 4% of the cosmic carbon available. On a galactic scale, the strength of the 3.4 microns band does not scale linearly with visual extinction, but instead increases more rapidly for objects near the Galactic Center. A similar trend is noted in the strength of the Si-O absorption band near 9.7 microns. The similar behavior of the C-H and Si-O stretching bands suggests that these two components may be coupled, perhaps in the form of grains with silicate cores and refractory organic mantles. The ubiquity of the hydrocarbon features seen in the near infrared near 3.4 microns throughout out Galaxy and in other galaxies demonstrates the widespread availability of such material for incorporation into the many newly forming planetary systems. The similarity of the 3.4 microns features in any organic material with aliphatic hydrocarbons underscores the need for complete astronomical observational coverage in the 2-30 microns region, of lines of sight which sample dust in both dense and diffuse interstellar clouds, in order to uniquely specify the composition of interstellar organics. This paper reviews the information available from ground-based observations, although currently the Infrared Satellite Observatory is adding to our body of knowledge on this subject by providing more extensive wavelength coverage. The Murchison carbonaceous meteorite has also been used as an analog to the interstellar observations and has revealed a striking similarity between the light hydrocarbons in the meteorite and the ISM; therefore this review includes comparisons with the meteoritic analog as well as with relevant laboratory residues. Fundamental to the evolution of the biogenic molecules, to the process of planetary system formation, and perhaps to the origin of life, is the connection between the organic material found in the interstellar medium and that incorporated in the most primitive solar system bodies.

Astronomy↗
PubMed1989

Chemical evolution of primitive solar system bodies.

In this paper we summarize some of the most salient observations made recently on the organic molecules and other compounds of the biogenic elements present in the interstellar medium and in the primitive bodies of the solar system. They include the discovery of the first phosphorus molecular species in dense interstellar clouds, the presence of complex organic ions in the dust and gas phase of Halley's coma, the finding of unusual, probably presolar, deuterium-hydrogen ratios in the amino acids of carbonaceous chondrites, and new developments on the chemical evolution of Titan, the primitive Earth, and early Mars. Some of the outstanding problems concerning the synthesis of organic molecules on different cosmic bodies are also discussed from an exobiological perspective.

Amino Acids↗
PubMedDate not supplied

Interstellar ices as a source of CN-bearing molecules in protoplanetary disks.

A reliable model for the composition and evolution of interstellar ices in regions of active star formation is fundamental to our quest to determine the organic inventory of planetesimals in the early Solar System. This has become a realistic goal since the launch of the Infrared Space Observatory, which provides a facility for infrared spectroscopy unhindered by telluric absorption over the entire spectral range of vibrational modes in solids of exobiological interest. Interstellar molecules detected in the solid phase to date include H2O, NH3, CO, CO2, CH3OH, CH4, H2CO, OCS and HCOOH, together with a C identical to N-bonded absorber generically termed 'XCN'. In this article, we focus on cosmic synthesis of CN-bearing species, as this important class of prebiotic molecules may not have formed endogenously in significant quantities on early Earth if conditions were not highly reducing. Experiments in which interstellar ice analogs are subject to UV photolysis or energetic ion bombardment yield CN-rich residues with a spectral signature that matches a corresponding feature observed in young protostars enshrouded in dust and gas. CN-bearing species are also present in cometary ices, with a combined abundance comparable to the lower end of the range observed in protostars. Energetic processing of interstellar ices is thus a viable and potentially significant source of CN compounds in protoplanetary disks.

Evolution, Chemical↗
PubMed2005

A large population of galaxies 9 to 12 billion years back in the history of the Universe.

To understand the evolution of galaxies, we need to know as accurately as possible how many galaxies were present in the Universe at different epochs. Galaxies in the young Universe have hitherto mainly been identified using their expected optical colours, but this leaves open the possibility that a significant population remains undetected because their colours are the result of a complex mix of stars, gas, dust or active galactic nuclei. Here we report the results of a flux-limited I-band survey of galaxies at look-back times of 9 to 12 billion years. We find 970 galaxies with spectroscopic redshifts between 1.4 and 5. This population is 1.6 to 6.2 times larger than previous estimates, with the difference increasing towards brighter magnitudes. Strong ultraviolet continua (in the rest frame of the galaxies) indicate vigorous star formation rates of more than 10-100 solar masses per year. As a consequence, the cosmic star formation rate representing the volume-averaged production of stars is higher than previously measured at redshifts of 3 to 4.

Journal Article↗
PubMed1991

The interstellar C-H stretching band near 3.4 microns: constraints on the composition of organic material in the diffuse interstellar medium.

To better constrain and quantify the composition of material in the diffuse interstellar medium (ISM), absorption spectra between 3600 and 2700 cm-1 (2.8 and 3.7 microns) have been taken of objects which have widely varying amounts of visual extinction along different lines of sight. The spectra of these objects contain a broad feature centered at approximately 3300 cm-1 (approximately 3.0 microns), attributed to O-H stretching vibrations, and/or a feature near 2950 cm-1 (3.4 microns) attributed to C-H stretching vibrations. The lack of correlation between the strengths of these two bands indicates that they do not arise from the same molecular carrier. The features in the 3100-2700 cm-1 (3.2-3.7 microns) region fall into one of two classes. We attribute the first class of features to material in the diffuse ISM on the basis of the similarity between the band profiles along the very different lines of sight to Galactic center source IRS 7 and VI Cygni #12. Similar features are also reported for Galactic center source IRS 3, Ve 2-45, and AFGL 2179. Higher resolution spectra of the objects OH 01-477 and T629-5, which are known to be M stars, are dominated by a series of narrow bands in this region. These bands are largely due to OH in the stars' photospheres. While the spectra of OH 01-477 and T629-5 are likely to contain C-H absorption from diffuse ISM dust, the strength of the overlapping photospheric OH features presently prevents us from quantifying the depths of the interstellar C-H feature towards these objects. The interstellar feature for Galactic center source IRS 7 has subpeaks near 2955, 2925, and 2870 cm-1 (+/- 5 cm-1), which we attribute to C-H stretching vibrations in the -CH2- and -CH3 groups of aliphatic hydrocarbons. These band positions fall within 5 cm-1 of the values normal for saturated aliphatics. The absence of a distinct band near 2855 cm-1 suggests that the material contains small amounts of electronegative groups like -O-H or -C triple bond N. The relative strengths and profiles of the 2955 and 2925 cm-1 features towards five objects suggests an average diffuse ISM line-of-sight -CH2-/-CH3 ratio of about 2.5, indicating the presence of relatively complex organic materials. The strengths of the subpeaks at 2925 and 2955 cm-1, due to -CH2- and -CH3 groups, respectively, correlate with visual extinction, strongly suggesting that the C-H stretching band is a general feature of the material along different lines of sight in the diffuse ISM. We find average ratios of A nu/tau(2925 cm-1) = 240 +/- 40 and A nu/tau(2955 cm-1) = 310 +/- 90 for the objects we have observed. We deduce that 2.6%-35% of the cosmic carbon in the ISM is tied up in the carrier of this band with the most likely value falling near 10%. The interstellar C-H band is remarkably similar to the feature in lab residues produced by irradiating analogs of dense molecular cloud ices. This is consistent with a model in which the hydrocarbon component in the diffuse interstellar medium consists of complex hydrocarbons containing aliphatic side chains and bridges which are produced in dense molecular clouds and subsequently modified in the diffuse medium.

Astronomical Phenomena↗
PubMed1997

The determination of ice composition with instruments on cometary landers.

The determination of the composition of materials that make up comets is essential in trying to understand the origin of these primitive objects. The ices especially could be made in several different astrophysical settings including the solar nebula, protosatellite nebulae of the giant planets, and giant molecular clouds that predate the formation of the solar system. Each of these environments makes different ices with different composition. In order to understand the origin of comets, one needs to determine the composition of each of the ice phases. For example, it is of interest to know that comets contain carbon monoxide, CO, but it is much more important to know how much of it is a pure solid phase, is trapped in clathrate hydrates, or is adsorbed on amorphous water ice. In addition, knowledge of the isotopic composition of the constituents will help determine the process that formed the compounds. Finally, it is important to understand the bulk elemental composition of the nucleus. When these data are compared with solar abundances, they put strong constraints on the macro-scale processes that formed the comet. A differential scanning calorimeter (DSC) and an evolved gas analyzer (EGA) will make the necessary association between molecular constituents and their host phases. This combination of instruments takes a small (tens of mg) sample of the comet and slowly heats it in a sealed oven. As the temperature is raised, the DSC precisely measures the heat required, and delivers the gases to the EGA. Changes in the heat required to raise the temperature at a controlled rate are used to identify phase transitions, e.g., crystallization of amorphous ice or melting of hexagonal ice, and the EGA correlates the gases released with the phase transition. The EGA consists of two mass spectrometers run in tandem. The first mass spectrometer is a magnetic-sector ion-momentum analyzer (MAG), and the second is an electrostatic time-of-flight analyzer (TOF). The TOF acts as a detector for the MAG and serves to resolve ambiguities between fragments of similar mass such as CO and N2. Because most of the compounds of interest for the volatile ices are simple, a gas chromatograph is not needed and thus more integration time is available to determine isotopic ratios. A gamma-ray spectrometer (GRS) will determine the elemental abundances of the bulk cometary material by determining the flux of gamma rays produced from the interaction of the cometary material with cosmic ray produced neutrons. Because the gamma rays can penetrate a distance of several tens of centimeters a large volume of material is analyzed. The measured composition is, therefore, much more likely to be representative of the bulk comet than a very small sample that might have lost some of its volatiles. Making these measurements on a lander offers substantial advantages over trying to address similar objectives from an orbiter. For example, an orbiter instrument can determine the presence and isotopic composition of CO in the cometary coma, but only a lander can determine the phase(s) in which the CO is located and separately determine the isotopic composition of each reservoir of CO. The bulk composition of the nucleus might be constrained from separate orbiter analyses of dust and gas in the coma, but the result will be very model dependent, as the ratio of gas to dust in the comet will vary and will not necessarily be equal to the bulk value.

Ammonia↗
PubMed2004

MEP (Mars Environment Package): toward a package for studying environmental conditions at the surface of Mars from future lander/rover missions.

In view to prepare Mars human exploration, it is necessary to promote and lead, at the international level, a highly interdisciplinary program, involving specialists of geochemistry, geophysics, atmospheric science, space weather, and biology. The goal of this program will be to elaborate concepts of individual instruments, then of integrated instrumental packages, able to collect exhaustive data sets of environmental parameters from future landers and rovers of Mars, and to favour the conditions of their implementation. Such a program is one of the most urgent need for preparing human exploration, in order to develop mitigation strategies aimed at ensuring the safety of human explorers, and minimizing risk for surface operations. A few main areas of investigation may be listed: particle and radiation environment, chemical composition of atmosphere, meteorology, chemical composition of dust, surface and subsurface material, water in the subsurface, physical properties of the soil, search for an hypothesized microbial activity, characterization of radio-electric properties of the Martian ionosphere. Scientists at the origin of the present paper, already involved at a high degree of responsibility in several Mars missions, and actively preparing in situ instrumentation for future landed platforms (Netlander--now cancelled, MSL-09), express their readiness to participate in both ESA/AURORA and NASA programs of Mars human exploration. They think that the formation of a Mars Environment working group at ESA, in the course of the AURORA definition phase, could act positively in favour of the program, by increasing its scientific cross-section and making it still more focused on human exploration.

Atmosphere↗