PubMed · 10857597
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D Bradley. 2000-06-01. Problematic standards.. https://doi.org/10.1021/ac002836q
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Organophosphate esters (OPEs), widely used as flame retardants and plasticizers, have been increasingly detected in aquatic environments. However, investigations of their distribution in high-altitude plateau lakes remain scarce. Identifying and quantifying the sources and associated risks of OPEs are crucial for subsequent water environment management. In this study, an integrated source-risk analysis approach was employed by combining the Positive Matrix Factorization (PMF) model, the Geodetector (GD) model, and risk quotient (RQ). Analysis of 14 OPEs in surface waters of the Dianchi Lake Basin (DLB) revealed 12 detectable compounds, with total OPEs concentrations (ΣOPEs) ranging from not detected (ND)-64.6 ng/L during the wet season and ND-35.8 ng/L during the dry season. Elevated ΣOPEs were primarily observed at inflow sites in the northern part of the lake and in urban rivers. Source apportionment indicated four major contributing sources: agricultural films containing flame-retardant and plasticizer additives, traffic-related particulate emissions, releases from household and personal care products, and industrial production and applications of flame retardants in plastics, electronics, and related products (the predominant source). The ecological impact caused by OPEs ranges from no risk to low risk, with tris(2-chloroethyl) phosphate emitted from industrial source being the primary driver of potential environmental risk. These findings highlight the necessity of prioritizing industrial sources in future management strategies. Overall, this study provides a methodological framework for source apportionment and risk assessment of OPEs and offers scientific evidence to support environmental management of OPEs in the DLB.
Hydrochemical data from catchment streams at three Environmental Change Network (ECN) upland catchments in north-east Scotland, south-east Scotland and northern England have been subjected to statistical analysis to separate the components due to long-term trend, season and flow. The relative variances due to each are presented for pH, Ca, SO4-S, NO3-N, DOC and Cl. Long-term trends have been identified with increases in concentration for NO3-N and DOC, decreases in SO4-S concentrations, along with short-term seasonal fluctuations. Application of this trend technique has allowed the detection of changes and contributed to an improved understanding of catchment behaviour.
Water quality in Scotland has progressively improved over the past 50 years as the environmental damage, which resulted from the industrial revolution, has been addressed. This paper provides an overview of current water quality in rivers, lochs, estuaries and coastal waters and describes the limited information available on groundwater. The main factors affecting water quality are reviewed, with sewage, diffuse agricultural pollution, acidification and urban drainage identified as the most important. Trends in pollution pressure and levels of investment in pollution control have been used to predict the condition of Scotland's surface water over the next 10 years. Major improvements are expected. However, progress will be slowed by the increased relative importance of diffuse sources of pollution, which are less amenable to legislative controls. Future changes in environmental monitoring are also expected to move the emphasis away from point source pollution. The current freshwater classification schemes are based upon a relatively narrow measure of water quality and are expected to expand to include a wider range of ecological parameters. This will result in an increase in the waters defined as impacted as the effects of other environmental pressures are taken into account. Finally the implications of these changes for the future management of the aquatic environment are assessed.