Zoe-Elizabeth Sariyanni | Search PubMed

PubMed2006

Electromagnetically induced coherent backscattering.

We demonstrate a strong coherent backward wave oscillation using forward propagating fields only. This is achieved by applying laser fields to an ultradispersive medium with proper chosen detunings to excite a molecular vibrational coherence that corresponds to a backward propagating wave. The physics then has much in common with the propagation of ultraslow light. Applications to coherent scattering and remote sensing are discussed.

Journal Article↗

PubMed2005

Visible and UV coherent Raman spectroscopy of dipicolinic acid.

We use time-resolved coherent Raman spectroscopy to obtain molecule-specific signals from dipicolinic acid (DPA), which is a marker molecule for bacterial spores. We use femtosecond laser pulses in both visible and UV spectral regions and compare experimental results with theoretical predictions. By exciting vibrational coherence on more than one mode simultaneously, we observe a quantum beat signal that can be used to extract the parameters of molecular motion in DPA. The signal is enhanced when an UV probe pulse is used, because its frequency is near-resonant to the first excited electronic state of the molecule. The capability for unambiguous identification of DPA molecules will lead to a technique for real-time detection of spores.

Biomarkers↗