Search PubMed⌕ Search

Biomedical subjects

X W Tu

Publications and source records attributed to X W Tu.

2 recordsLinked to original sources

Atomic scale control of single molecule charging.

A scanning tunneling microscope was used to study charging of single copper phthalocyanine molecules adsorbed on an ultrathin Al(2)O(3) film grown on a NiAl(110) surface. A double-barrier tunnel junction is formed by a vacuum barrier between the tip and the molecule and an oxide barrier between the molecule and the NiAl. In this geometry the molecule can be charged by the tunneling electrons. This charging was found to be strongly dependent on the position of the tip above the molecule and the applied bias voltage.

Journal Article↗

Atomic-scale rectification at microwave frequency.

Microwave of known amplitude and frequency, irradiating the junction of a low temperature scanning tunneling microscope, was found to induce a dc signal. This rectification current is spatially localized and exhibits chemical sensitivity at the atomic scale. Dependence of the rectification current on the sample bias voltage reveals spin splitting in the electronic state of a single Mn atom and vibrations of single MnCO molecule. These results demonstrate the feasibility of atomic scale nonlinear spectroscopy and the potential for the detection of resonance phenomena excited with a spatially extended electromagnetic wave.

Journal Article↗