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P Verkerk

Publications and source records attributed to P Verkerk.

At least 19 recordsLinked to original sources

How well do we know atomic motions of simple liquids?

Microscopic motions in molten potassium spanning three frequency decades are studied by neutron-scattering techniques. These comprise well-defined density oscillations and stochastic particle rearrangements and both are modeled on microscopic grounds. While vibratory motions are shown to share characteristics with those of their parent crystals, dynamic correlations between a diffusing particle and its neighbors can be accounted for only semiquantitatively.

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Neutron Brillouin scattering study of collective dynamics in a dense He-Ne gaseous mixture.

The dynamic structure factor S(k,omega) of a 77% He and 23% Ne gaseous mixture at T = 39.3 K and total number density n = 15.8 nm(-3) has been measured by inelastic neutron scattering at small angles. In the range of wave vectors studied, 0.7<k/nm(-1)<1.8, we find clear side peaks at frequencies following the hydrodynamic sound dispersion c k of the binary mixture (with c the adiabatic sound speed in the mixture). Surprisingly, neither fast modes nor a transition from normal to fast sound are observed in the above low- k region, indicating that hydrodynamic behavior persists up to k values which are larger than those predicted by theories and computer simulations.

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Quantum effects on liquid dynamics as evidenced by the presence of well-defined collective excitations in liquid para-hydrogen

The origin of the well-defined collective excitations found in liquid para-H2 by recent experiments is investigated. The persistence of their relatively long lifetimes down to microscopic scales is well accounted for by calculations carried out by means of path-integral-centroid molecular dynamics. In contrast only overdamped excitations are found in calculations carried within the classical limit. The results provide fully quantitative evidence of quantum effects on the dynamics of a simple liquid.

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