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M Imlau

Publications and source records attributed to M Imlau.

7 recordsLinked to original sources
PubMed2006

Evidence for two-path recombination of photoinduced small polarons in reduced LiNbO(3).

The recombination of photoinduced free Nb(4+)(Nb) and bound Nb(4+)(Li) small polarons toNb(4+)(Li): Nb(4+)(Nb) bipolarons is investigated in nominally pure, reduced LiNbO(3) single crystals by means of excited-state-absorption spectroscopy. We discovered a two-component decay of the light-induced absorption alpha(li)(t) for probe light at lambda=785 nm and moderate pump beam intensities (I(p) << 670 GW/m(2)). These experimental results give strong evidence for the existence of a two-path recombination of the photoinduced polarons. A corresponding model taking into account hopping charge transport and trapping is presented.

Journal Article↗
PubMed2005

Evidence for light-induced hole polarons in LiNbO3.

Transient light-induced absorption in LiNbO3 is observed in the blue-green spectral range after pulsed illumination with 532 nm. Its buildup and decay in Fe-doped LiNbO3 is satisfactorily described by a sum of two stretched exponential functions. For undoped LiNbO3, however, only one stretched exponential decay is observed. These experimental results are explained by the formation of both small Nb(Li)4+ electron polarons and O- hole polarons. The mechanism is discussed on the basis of a proposed band scheme.

Journal Article↗
PubMed2005

Comment on "Theoretical study of the photoinduced transfer among the ground state and two metastable states in [Fe(CN)5NO]2-" [J. Chem. Phys. 122, 074314 (2005)].

We discuss the computational results of the "Theoretical study of the photoinduced transfer among the ground state and two metastable states in [Fe(CN)5NO]2-" [J. Chem. Phys. 122, 074314 (2005)] with respect to our previously reported polarized absorption study on the metastable states SI and SII in Na2[Fe(CN)5NO]2H2O [D. Schaniel, J. Schefer, B. Delley, M. Imlau, and Th. Woike, Phys. Rev. B 66, 085103 (2002)].

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PubMed2004

Change from 3D-Ising to random field-Ising-model criticality in a uniaxial relaxor ferroelectric.

Pyroelectric measurements of polarization have been used to determine the temperature dependence of the polarization in strontium barium niobate, SBN:Ce, close to its phase transition temperature T(c) approximately 317 K. A gradual increase of the critical exponent from beta approximately 0.13 to beta approximately 0.30 is observed when decreasing the initial polarization from 100% to 0.8% of the saturation value. A change from three-dimensional random-field Ising to pure Ising model behavior is conjectured and explained by a gradual compensation of quenched random electric fields by those emerging from charged fractal nanodomain walls.

Journal Article↗
PubMed2003

New parametric scattering in photorefractive Sr0.61Ba0.39Nb2O6:Cr.

A new class of light-induced parametric scattering, not included in the conventional model, has been discovered in photorefractive Sr(0.61)Ba(0.39)Nb(2)O(6):Cr illuminated by two coherent beams. A novel model of multiwave mixing of coherent noise and transmitted light is developed to explain the new scattering phenomena. The model includes all known types and predicts a multitude of new types of parametric scattering. Generalized phase-matching conditions for parametric scattering in photorefractive crystals are proposed.

Journal Article↗
PubMed2002

Polarization-based adjustable memory behavior in relaxor ferroelectrics.

The irreversible decay of the spontaneous polarization above the phase-transition temperature is a limiting factor in any application of ferroelectric crystals. Here we show that electric fields applied at high temperatures induce a preferred direction in the crystal which is stable even after repeated heating and cooling through the phase transition. This preference in direction leads to a reorientation of domains in the ferroelectric phase. We use pyroelectric measurements to show that the directional preference originates from internal charge carriers interacting with domain walls.

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