Search PubMed⌕ Search

Biomedical subjects

J-P Bouchaud

Publications and source records attributed to J-P Bouchaud.

7 recordsLinked to original sources

Direct experimental evidence of a growing length scale accompanying the glass transition.

Understanding glass formation is a challenge, because the existence of a true glass state, distinct from liquid and solid, remains elusive: Glasses are liquids that have become too viscous to flow. An old idea, as yet unproven experimentally, is that the dynamics becomes sluggish as the glass transition approaches, because increasingly larger regions of the material have to move simultaneously to allow flow. We introduce new multipoint dynamical susceptibilities to estimate quantitatively the size of these regions and provide direct experimental evidence that the glass formation of molecular liquids and colloidal suspensions is accompanied by growing dynamic correlation length scales.

Journal Article↗

Spin anisotropy and slow dynamics in spin glasses.

We report on an extensive study of the influence of spin anisotropy on spin glass aging dynamics. New temperature cycle experiments allow us to compare quantitatively the memory effect in four Heisenberg spin glasses with various degrees of random anisotropy and one Ising spin glass. The sharpness of the memory effect appears to decrease continuously with the spin anisotropy. Besides, the spin glass coherence length is determined by magnetic field change experiments for the first time in the Ising sample. For three representative samples, from Heisenberg to Ising spin glasses, we can consistently account for both sets of experiments (temperature cycle and magnetic field change) using a single expression for the growth of the coherence length with time.

Journal Article↗

Linear and nonlinear response in the aging regime of the one-dimensional trap model.

We investigate the behavior of the response function in the one-dimensional trap model using scaling arguments that we confirm by numerical simulations. We study the average position of the random walk at time t(w)+t, given that a small bias h is applied at time t(w). Several scaling regimes are found, depending on the relative values of t, t(w), and h. Comparison with the diffusive motion in the absence of bias allows us to show that the fluctuation-dissipation relation is valid even in the aging regime, at least for times such that linear response is obeyed. However, for sufficiently long times, the response always becomes nonlinear in h.

Journal Article↗

Statistical aging and nonergodicity in the fluorescence of single nanocrystals.

The relation between single particle and ensemble measurements is addressed for semiconductor CdSe nanocrystals. We record their fluorescence at the single molecule level and analyze their emission intermittency, which is governed by unusual random processes known as Lévy statistics. We report the observation of statistical aging and ergodicity breaking, both related to the occurrence of Lévy statistics. Our results show that the behavior of ensemble quantities, such as the total fluorescence of an ensemble of nanocrystals, can differ from the time-averaged individual quantities, and must be interpreted with care.

Cadmium Compounds↗

Anisotropy in granular media: classical elasticity and directed-force chain network.

A general approach is presented for understanding the stress response function in anisotropic granular layers in two dimensions. The formalism accommodates both classical anisotropic elasticity theory and linear theories of anisotropic directed-force chain networks. Perhaps surprisingly, two-peak response functions can occur even for classical, anisotropic elastic materials, such as triangular networks of springs with different stiffnesses. In such cases, the peak widths grow linearly with the height of the layer, contrary to the diffusive spreading found in "stress-only" hyperbolic models. In principle, directed-force chain networks can exhibit the two-peak, diffusively spreading response function of hyperbolic models, but all models in a particular class studied here are found to be in the elliptic regime.

Journal Article↗

Subdiffusion and localization in the one-dimensional trap model.

We study a one-dimensional generalization of the exponential trap model using both numerical simulations and analytical approximations. We obtain the asymptotic shape of the average diffusion front in the subdiffusive phase. Our central result concerns the localization properties. We find the dynamical participation ratios to be finite, but different from their equilibrium counterparts. Therefore, the idea of a partial equilibrium within the limited region of space explored by the walk is not exact, even for long times where each site is visited a very large number of times. We discuss the physical origin of this discrepancy, and characterize the full distribution of dynamical weights. We also study two different two-time correlation functions, which exhibit different aging properties: one is "sub aging" whereas the other one shows "full aging," therefore, two diverging time scales appear in this model. We give intuitive arguments and simple analytical approximations that account for these differences, and obtain new predictions for the asymptotic (short-time and long-time) behavior of the scaling functions. Finally, we discuss the issue of multiple time scalings in this model.

Journal Article↗

Anomalous dynamical light scattering in soft glassy gels.

We compute the dynamical structure factor S( q,tau) of an elastic medium where force dipoles appear at random in space and in time, due to "micro-collapses" of the structure. Various regimes are found, depending on the wave vector q and the collapse time theta. In an early time regime, the logarithm of the structure factor behaves as (q tau)(3/2), as predicted in (L. Cipelletti et al., Phys. Rev Lett. 84, 2275 (2000)) using heuristic arguments. However, in an intermediate-time regime we rather obtain a (q tau)(5/4) behaviour. Finally, the asymptotic long-time regime is found to behave as q(3/2)tau. We also give a plausible scenario for aging, in terms of a strain-dependent energy barrier for micro-collapses. The relaxation time is found to grow with the age t(w), quasi-exponentially at first, and then as t(w)(4/5) with logarithmic corrections.

Journal Article↗