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H Schulte-Schrepping

Publications and source records attributed to H Schulte-Schrepping.

9 recordsLinked to original sources

Observation of structural anisotropy and the onset of liquidlike motion during the nonthermal melting of InSb.

The melting dynamics of laser excited InSb have been studied with femtosecond x-ray diffraction. These measurements observe the delayed onset of diffusive atomic motion, signaling the appearance of liquidlike dynamics. They also demonstrate that the root-mean-squared displacement in the [111] direction increases faster than in the [110] direction after the first 500 fs. This structural anisotropy indicates that the initially generated fluid differs significantly from the equilibrium liquid.

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Atomic-scale visualization of inertial dynamics.

The motion of atoms on interatomic potential energy surfaces is fundamental to the dynamics of liquids and solids. An accelerator-based source of femtosecond x-ray pulses allowed us to follow directly atomic displacements on an optically modified energy landscape, leading eventually to the transition from crystalline solid to disordered liquid. We show that, to first order in time, the dynamics are inertial, and we place constraints on the shape and curvature of the transition-state potential energy surface. Our measurements point toward analogies between this nonequilibrium phase transition and the short-time dynamics intrinsic to equilibrium liquids.

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Clocking femtosecond X rays.

Linear-accelerator-based sources will revolutionize ultrafast x-ray science due to their unprecedented brightness and short pulse duration. However, time-resolved studies at the resolution of the x-ray pulse duration are hampered by the inability to precisely synchronize an external laser to the accelerator. At the Sub-Picosecond Pulse Source at the Stanford Linear-Accelerator Center we solved this problem by measuring the arrival time of each high energy electron bunch with electro-optic sampling. This measurement indirectly determined the arrival time of each x-ray pulse relative to an external pump laser pulse with a time resolution of better than 60 fs rms.

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Beam-position monitors in the X-ray undulator beamline at PETRA.

At the 12 GeV storage ring PETRA, the first synchrotron radiation beamline uses a 4 m-long undulator. The beamline, with a length of 130 m between source and sample, delivers hard X-ray photons usable up to 300 keV. The photon beam has a total power of 7 kW. Combined with the high brilliance, the powerful beam is very critical for all beamline components. Copper, located at a distance of 26 m, hit by the full undulator beam, melts within 20 ms. Different monitors are described for stable, safe and reliable operation of beam and experiments.

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Adaptive indirectly cooled monochromator crystals at HASYLAB.

The high-heat-load monochromator, based on the HASYLAB (Hamburger Synchrotronstrahlungslabor) 'Torii' design, has been used successfully for 2 years at the BW2 wiggler beamline. The bowing of the reflecting surface induced by the heat load and water pressure is compensated mechanically. This is achieved by mounting the specially shaped crystal in a bending mechanism and by heat transfer from the directly water-cooled crystal. We present the latest step in the development of this design. The piezoceramic-driven actuators are replaced by actuators based on the thermal expansion of copper rods. The direct water cooling of the crystal is replaced by a safer indirect water-cooling scheme. Characterization results of the crystal are presented. The Si(111) rocking-curve width at 9.5 keV was measured to be 8.3 arcsec under 500 W heat load.

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Measurements of emittance and absolute spectral flux of the PETRA undulator at DESY Hamburg.

The first synchrotron radiation beamline using a 4 m-long undulator at the 12 GeV storage ring PETRA delivers hard X-ray photons usable up to 300 keV. The photon intensity is measured on an absolute scale in the energy range between 16 and 60 keV and compared with calculated intensities. The experimental set-up described is also used to measure the horizontal and vertical emittance of the source.

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Adaptive Silicon Monochromators for High-Power Insertion Devices. Tests at CHESS, ESRF and HASYLAB.

X-ray wigglers which produce tens of kilowatts of photon power within the white beam will soon become available at third-generation sources of synchrotron radiation. Insertion devices that produce several kilowatts already exist and we have used those at CHESS, ESRF and HASYLAB to test adaptive 111 silicon water-jet-cooled monochromators at up to 2 kW total incident beam power. This development from earlier work at the Brookhaven National Synchrotron Light Source (NSLS) uses the pressure in the water coolant to provide active compensation of the strain field in the thermal footprint, nulling its effect to within residual variations in Bragg angle of only a few arc s. The design is robust, vacuum compatible and uses no moving mechanical parts.

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