Biomedical subjects

G Marowsky

Publications and source records attributed to G Marowsky.

11 recordsLinked to original sources

PubMed2005

Surface-enhanced optical third-harmonic generation in Ag island films.

Surface-enhanced optical third-harmonic generation (THG) is observed in silver island films. The THG intensity from Ag nanoparticles is enhanced by more than 2 orders of magnitude with respect to the THG intensity from a smooth and homogeneous silver surface. This enhancement is attributed to a local plasmon excitation and resonance of the local field at the third-harmonic wavelength. The diffuse and depolarized component of the enhanced THG is associated with the third-order hyper-Rayleigh scattering in a two-dimensional random array of silver nanoparticles.

Journal Article↗

PubMed2004

Enhanced two-photon fluorescence excitation by resonant grating waveguide structures.

Enhanced two-photon fluorescence (TPF) spectroscopy with novel high-finesse resonant polymeric grating waveguide structures (GWSs) is presented. Under resonant conditions the field enhancement at the surface of a GWS can be exploited for TPF spectroscopy without the need for highly focused laser excitation light. We compare the TPF obtained by placing a drop of tetramethylrhodamine (TMR) on top of a GWS with that obtained with TMR on top of a glass substrate. Our procedure and results indicate that the detection of TPF can be improved by a factor of 10 with resonant GWSs.

Equipment Design↗

PubMed2004

Ferroelectric ordering and electroclinic effect in chiral smectic liquid crystals.

Ferroelectric ordering, the electroclinic effect, and chiral smectic C(SmC*)-smectic A phase transitions in thin planar ferroelectric liquid crystal (FLC) cells are studied by means of linear electro-optic and second harmonic generation (SHG) techniques. The ferroelectric switching is detected in biased FLC cells by measuring azimuthal dependences of linear and nonlinear responses. The applied dc electric field rotates the FLC symmetry axis with initial and final orientations in the cell plane. Comparative studies of the SHG switching behavior in reflection and transmission geometries allows one to distinguish the contributions from the bulk and the subsurface layers of the cell. The analysis of SHG temperature dependences shows the existence of a strong surface coupling. The temperature-dependent nonlinear polarization shows a critical behavior with the exponent approximately 0.3 in SmC* phase.

Journal Article↗

PubMed2003

Two-photon fluorescence excitation of macroscopic areas on planar waveguides.

In this paper, we report the first successful demonstration, to our knowledge, of two-photon fluorescence excitation (TPFE) using planar thin-film waveguide structures of macroscopic excitation dimensions (square millimeters to square centimeters in size). The high intensity of excitation light required for TPFE is available not only at a single focus point but along the whole trace of the beam guided in the waveguide structure. Line profiles of the fluorescence excited by TPFE show excellent correlation with the geometry of the launched laser beams. A clear second-order dependence of the fluorescence intensity on the excitation intensity confirms the two-photon character of fluorescence generation. Spectra of the emission generated by one-photon excitation and by two-photon excitation show only minor differences.

Equipment Design↗

PubMed1994