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Biomedical subjects

D Charalambidis

Publications and source records attributed to D Charalambidis.

16 recordsLinked to original sources

Second order autocorrelation of an XUV attosecond pulse train.

Temporal widths of an attosecond (asec) XUV radiation pulse train, formed by the superposition of higher order harmonics, have been recently determined utilizing a 2nd order autocorrelation measurement. An assessment of the validity of the approach, for the broadband XUV radiation of asec pulses, is implemented through ab initio calculations modeling the spectral and temporal response of the two-XUV-photon He ionization detector employed. The measured width of the asec bursts is discussed in terms of the spectral phases of the individual harmonics, as well as in terms of the spatially modulated temporal width of the radiation, and is found in reasonable agreement with the expected duration.

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Direct observation of attosecond light bunching.

Temporal probing of a number of fundamental dynamical processes requires intense pulses at femtosecond or even attosecond (1 as = 10(-18) s) timescales. A frequency 'comb' of extreme-ultraviolet odd harmonics can easily be generated in the interaction of subpicosecond laser pulses with rare gases: if the spectral components within this comb possess an appropriate phase relationship to one another, their Fourier synthesis results in an attosecond pulse train. Laser pulses spanning many optical cycles have been used for the production of such light bunching, but in the limit of few-cycle pulses the same process produces isolated attosecond bursts. If these bursts are intense enough to induce a nonlinear process in a target system, they can be used for subfemtosecond pump-probe studies of ultrafast processes. To date, all methods for the quantitative investigation of attosecond light localization and ultrafast dynamics rely on modelling of the cross-correlation process between the extreme-ultraviolet pulses and the fundamental laser field used in their generation. Here we report the direct determination of the temporal characteristics of pulses in the subfemtosecond regime, by measuring the second-order autocorrelation trace of a train of attosecond pulses. The method exhibits distinct capabilities for the characterization and utilization of attosecond pulses for a host of applications in attoscience.

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Two-Photon Ionization of He through a Superposition of Higher Harmonics.

We present experimental results and theoretical analysis of two-photon ionization of He by a superposition of the 7th to the 13th harmonic of a Ti:sapphire laser. Solving the time-dependent Schrödinger equation for He in a coherent polychromatic field, the He+ yield is calculated. From this yield the number of He+ ions produced has been estimated and found in reasonable agreement with its measured value. The present results establish the feasibility of a second-order autocorrelation measurement of superposition of harmonics, and thus they represent the precursor towards the direct temporal characterization of attosecond pulse trains.

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Charge-state resolved above threshold ionization

Photoelectron energy resolved spectra recorded in coincidence with singly and doubly ionized atoms are reported for the interaction of xenon with 60 fs laser pulses at 800 nm and 1x10(14) W/cm(2). Double ionization contributions in the spectrum have been established. The appearance of a single ionization plateau in above threshold ionization is verified. A hotter electron distribution is found for the double ionization.

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